We report on the induction of magnetization in Rydberg systems by means of the inverse Faraday effect and propose the appearance of the effect in two such systems: Rydberg atoms proper and shallow dopants in semiconductors. Rydberg atoms are characterized by a large orbital radius. This large radius gives such excited states a large angular moment, which when driven with circularly polarized light translates to a large effective magnetic field Beff. We calculate this effect to generate effective magnetic fields of O(1μT)×(ω1THz)-1(I10Wcm-2)n4 in the Rydberg states of atoms such as Rb and Cs for off-resonant photon beams with frequency ω and intensity I expressed in units of the denominators and n the principal quantum number. Additionally, terahertz spectroscopy of phosphorus-doped silicon reveals a large cross section for excitation of shallow dopants to Rydberg-like states, which even for small n have the potential to be driven similarly with circularly polarized light to produce an even larger magnetization. Our theoretical calculations estimate Beff as O(102T) for Si:P with a beam intensity of 108Wcm-2.

The mobility edge (ME) is a crucial concept in understanding localization physics, marking the critical transition between extended and localized states in the energy spectrum. Anderson localization scaling theory predicts the absence of ME in lower dimensional systems. Hence, the search for exact MEs, particularly for single particles in lower dimensions, has recently garnered significant interest in both theoretical and experimental studies, resulting in notable progress. However, several open questions remain, including the possibility of a single system exhibiting multiple MEs and the continual existence of extended states, even within the strong disorder domain. Here, we provide experimental evidence to address these questions by utilizing a quasiperiodic mosaic lattice with meticulously designed nanophotonic circuits. Our observations demonstrate the coexistence of both extended and localized states in lattices with broken duality symmetry and varying modulation periods. By single-site injection and scanning the disorder level, we could approximately probe the ME of the modulated lattice. These results corroborate recent theoretical predictions, introduce a new avenue for investigating ME physics, and offer inspiration for further exploration of ME physics in the quantum regime using hybrid integrated photonic devices.

We propose to realize the quantum nonlinear Hall effect and the inverse Faraday effect through the acoustic wave in a time-reversal invariant but inversion broken Dirac insulator. We focus on the acoustic frequency much lower than the Dirac gap such that the interband transition is suppressed and these effects arise solely from the intrinsic valley-contrasting band topology. The corresponding acoustoelectric conductivity and magnetoacoustic susceptibility are both proportional to the quantized valley Chern number and independent of the quasiparticle lifetime. The linear and nonlinear components of the longitudinal and transverse topological currents can be tuned by adjusting the polarization and propagation directions of the surface acoustic wave. The static magnetization generated by a circularly polarized acoustic wave scales linearly with the acoustic frequency as well as the strain-induced charge density. Our results unveil a quantized nonlinear topological acoustoelectric response of gapped Dirac materials, like hexagonal boron nitride and transition-metal dichalcogenide, paving the way toward room-temperature acoustoelectric devices due to their large band gaps.

Recent experiments demonstrate precise control over coherently excited circular phonon modes using high-intensity terahertz lasers, opening new pathways towards dynamical, ultrafast design of magnetism in functional materials. While the phonon Zeeman effect enables a theoretical description of phonon-induced magnetism, it lacks efficient angular momentum transfer from the phonon to the electron sector. In this work, we put forward a coupling mechanism based on electron-nuclear quantum geometry, with the inverse Faraday effect as a limiting case. This effect is rooted in the phase accumulation of the electronic wave function under a circular evolution of nuclear coordinates. An excitation pulse then induces a transient level splitting between electronic orbitals that carry angular momentum. First-principles simulations on SrTiO3 demonstrate that in parts of the Brillouin zone, this splitting between orbitals carrying angular momentum can easily reach 50 meV.

We investigate the effects of a Laguerre-Gaussian (LG) beam on the superconducting state. We show that the vortex angular momentum of a LG beam affects the superconducting state and induces currents. The induction of the current by microwave radiation is illustrated on a Josephson loop and SQUID devices. In particular, we establish that coupling a dc SQUID to the ac magnetic flux of a LG beam can stabilize the π phase in the SQUID. This can happen via developing a global or local minimum in the effective potential at π. In the latter case, this happens via the Kapitza mechanism.

Dynamical perturbations modify the states of classical systems in surprising ways and give rise to important applications in science and technology. For example, Floquet engineering exploits the possibility of band formation in the frequency domain when a strong, periodic variation is imposed on parameters such as spring constants. We describe here Kapitza engineering, where a drive field oscillating at a frequency much higher than the characteristic frequencies for the linear response of a system changes the potential energy surface so much that maxima found at equilibrium become local minima, in precise analogy to the celebrated Kapitza pendulum where the unstable inverted configuration, with the mass above rather than below the fulcrum, actually becomes stable. Our starting point is a quantum field theory of the Ginzburg-Devonshire type, suitable for many condensed matter systems, including particularly ferroelectrics and quantum paralectrics. We show that an off-resonance oscillatory electric field generated by a laser-driven terahertz source can induce ferroelectric order in the quantum-critical limit. Heating effects are estimated to be manageable using pulsed radiation; "hidden"radiation-induced order can persist to low temperatures without further pumping due to stabilization by strain. We estimate the Ginzburg-Devonshire free-energy coefficients in SrTiO3 using density-functional theory and the stochastic self-consistent harmonic approximation accelerated by a machine-learned force field. Although we find that SrTiO3 is not an optimal choice for Kapitza stabilization, we show that scanning for further candidate materials can be performed at the computationally convenient density-functional theory level. We suggest second harmonic generation, soft-mode spectroscopy, and x-ray diffraction experiments to characterize the induced order.

We present a microscopic calculation of the inverse Faraday effect in metals. We derive a static local magnetic moment induced on the application of high-frequency light, using the Eilenberger formulation of quasiclassical theory. We include the effect of disorder and formulate a theory applicable across the entire temperature range, in the absence of external applied fields. For light-induced electric fields of amplitude ∼100kV/cm, the induced fields are large ∼0.1T for metallic Nb. The predictions of our theory agree with recent experimental and theoretical results [O. H.-C. Cheng, Nat. Photon. 14, 365 (2020)1749-488510.1038/s41566-020-0603-3 and J. Hurst, Phys. Rev. B 98, 134439 (2018)2469-995010.1103/PhysRevB.98.134439]. An extension of this approach to superconductors would open a new route of inducing orbital magnetic field and potentially vortices in superconductors.

The increasing financial and environmental cost of many inorganic materials has motivated study into organic and “green” alternatives. However, most organic compounds contain a large number of atoms in the primitive unit cell, posing a significant barrier to high-throughput screening for functional properties. In this work, we attempt to overcome this challenge and identify superconducting candidates among the metal-organic-frameworks in the organic materials database using a recently proposed proxy for the electron-phonon coupling. We then isolate the most promising candidate for in-depth analysis, C9H8Mn2O11, providing evidence for superconductivity below 100mK.

The application of dynamic strain holds the potential to manipulate topological invariants in topological quantum materials. This study investigates dynamic structural deformation and strain modulation in the Weyl semimetal WTe2, focusing on the microscopic regions with static strain defects. The interplay of static strain fields, at local line defects, with dynamic strain induced from photo-excited coherent acoustic phonons results in the formation of local standing waves at the defect sites. The dynamic structural distortion is precisely determined utilizing ultrafast electron microscopy with nanometer spatial and gigahertz temporal resolutions. Numerical simulations are employed to interpret the experimental results and explain the mechanism for how the local strain fields are transiently modulated through light-matter interaction. This research provides the experimental foundation for investigating predicted phenomena such as the mixed axial-torsional anomaly, acoustogalvanic effect, and axial magnetoelectric effects in Weyl semimetals, and paves the road to manipulate quantum invariants through transient strain fields in quantum materials.

Quantum transport and localization are fundamental concepts in condensed matter physics. It is commonly believed that in one-dimensional systems, the existence of mobility edges is highly dependent on disorder. Recently, there has been a debate over the existence of an exact mobility edge in a modulated mosaic model without quenched disorder, the so-called mosaic Wannier-Stark lattice. Here, we experimentally implement such disorder-free mosaic photonic lattices using a silicon photonics platform. By creating a synthetic electric field, we could observe energy-dependent coexistence of both extended and localized states in a finite number of waveguides. The Wannier-Stark ladder emerges when the resulting potential is strong enough, and can be directly probed by exciting different spatial modes of the lattice. Our studies provide the experimental proof of coexisting sets of strongly localized and conducting (though weakly localized) states in finite-sized mosaic Wannier-Stark lattices, which hold the potential to encode high-dimensional quantum resources with compact and robust structures.