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Across the Board: Licheng Sun on the Mechanism of O-O Bond Formation in Photosystem II
KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Chemistry.ORCID iD: 0000-0002-4093-1251
KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD. KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Chemistry, Organic chemistry. Dalian Univ Technol.ORCID iD: 0000-0002-4521-2870
2019 (English)In: ChemSusChem, ISSN 1864-5631, E-ISSN 1864-564X, Vol. 12, no 14, p. 3401-3404Article in journal (Refereed) Published
Abstract [en]

In this series of articles, the board members of ChemSusChem discuss recent research articles that they consider of exceptional quality and importance for sustainability. This entry features Prof. L. Sun, who proposes a special mechanism for O-O bond formation in photosystem II with involvement of an Mn-VII-oxo species induced by charge- and structural rearrangements. In this viewpoint, Proton transfer is involved in changes of the first coordination spheres around the Mn-VII-oxo site on the dangling Mn4 with de- and re-coordination of carboxylates (Glu333 and Asp170).

Place, publisher, year, edition, pages
WILEY-V C H VERLAG GMBH , 2019. Vol. 12, no 14, p. 3401-3404
Keywords [en]
disproportionation, oxygen evolution, photosystem II, structural rearrangement, water splitting
National Category
Biochemistry and Molecular Biology
Identifiers
URN: urn:nbn:se:kth:diva-257575DOI: 10.1002/cssc.201901438ISI: 000478633900023PubMedID: 31240851Scopus ID: 2-s2.0-85068351514OAI: oai:DiVA.org:kth-257575DiVA, id: diva2:1353362
Note

QC 20190923

Available from: 2019-09-23 Created: 2019-09-23 Last updated: 2019-09-23Bibliographically approved

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Zhang, BiaobiaoSun, Licheng

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