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Ultrafast dynamics of hole self-localization in beta-Ga2O3
KTH, School of Engineering Sciences (SCI), Applied Physics, Photonics.ORCID iD: 0000-0002-4606-4865
2020 (English)In: Applied Physics Letters, ISSN 0003-6951, E-ISSN 1077-3118, Vol. 116, no 13, article id 132101Article in journal (Refereed) Published
Abstract [en]

Hole self-localization into polaron states is a phenomenon characteristic of many wide bandgap compounds including transparent semiconducting oxide beta-Ga2O3. While this effect has been recognized for some time, its dynamics remained elusive, and self-localization has often been considered instantaneous. In this work, using the two-color ultrafast pump-probe technique, we have measured the hole self-localization time in beta-Ga2O3. At room temperature, this time has been found to be 0.5 ps increasing to 1.1 ps at 10K. In terms of the configuration coordinate diagram, at room temperature, tunneling and thermal activation contribute to the process with similar weights. The hole self-trapping coefficient is estimated to be 6.4x10(-8)cm(3)/s.

Place, publisher, year, edition, pages
AMER INST PHYSICS , 2020. Vol. 116, no 13, article id 132101
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Condensed Matter Physics
Identifiers
URN: urn:nbn:se:kth:diva-272634DOI: 10.1063/5.0003682ISI: 000523436000001Scopus ID: 2-s2.0-85082741138OAI: oai:DiVA.org:kth-272634DiVA, id: diva2:1429689
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QC 20200512

Available from: 2020-05-12 Created: 2020-05-12 Last updated: 2022-06-26Bibliographically approved

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Marcinkevičius, Saulius

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