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Dimensionality Modulates Electrical Conductivity in Compositionally Constant One-, Two-, and Three-Dimensional Frameworks
MIT, Dept Chem, Cambridge, MA 02139 USA..
MIT, Dept Chem, Cambridge, MA 02139 USA..
MIT, Dept Chem, Cambridge, MA 02139 USA..
MIT, Dept Chem, Cambridge, MA 02139 USA..
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2022 (English)In: Journal of the American Chemical Society, ISSN 0002-7863, E-ISSN 1520-5126, Vol. 144, no 12, p. 5583-5593Article in journal (Refereed) Published
Abstract [en]

We reveal here the construction of Ni-based metal-organic frameworks (MOFs) and conjugated coordination polymers (CCPs) with different structural dimensionalities, including closely pi-stacked 1D chains (Ni-1D), aggregated 2D layers (Ni-2D), and a 3D framework (Ni-3D), based on 2,3,5,6-tetraamino-1,4-hydroquinone (TAHQ) and its various oxidized forms. These materials have the same metal-ligand composition but exhibit distinct electronic properties caused by different dimensionalities and supramolecular interactions between SBUs, ligands, and structural motifs. The electrical conductivity of these materials spans nearly 8 orders of magnitude, approaching 0.3 S/cm.

Place, publisher, year, edition, pages
American Chemical Society (ACS) , 2022. Vol. 144, no 12, p. 5583-5593
National Category
Materials Chemistry
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URN: urn:nbn:se:kth:diva-313502DOI: 10.1021/jacs.2c00614ISI: 000799109400046PubMedID: 35290048Scopus ID: 2-s2.0-85127122662OAI: oai:DiVA.org:kth-313502DiVA, id: diva2:1665348
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QC 20220607

Available from: 2022-06-07 Created: 2022-06-07 Last updated: 2022-06-25Bibliographically approved

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Li, Jian

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