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Efficient perovskite LEDs with tailored atomic layer number emission at fixed wavelengths
KTH, School of Engineering Sciences (SCI), Applied Physics. Peking Univ, Sch Mat Sci & Engn, Beijing 100871, Peoples R China.;Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England.;Peking Univ, State Key Lab Rare Earth Mat Chem & Applicat, PKU HKU Joint Lab Rare Earth Mat & Bioinorgan Chem, Beijing Natl Lab Mol Sci,Coll Chem & Mol Engn, Beijing 100871, Peoples R China.ORCID iD: 0000-0003-4220-1161
Univ Cambridge, Dept Chem Engn & Biotechnol, Cambridge CB3 0AS, Cambs, England..
Peking Univ, State Key Lab Rare Earth Mat Chem & Applicat, PKU HKU Joint Lab Rare Earth Mat & Bioinorgan Chem, Beijing Natl Lab Mol Sci,Coll Chem & Mol Engn, Beijing 100871, Peoples R China..
Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England..
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2025 (English)In: Science Advances, E-ISSN 2375-2548, Vol. 11, no 7, article id eadp9595Article in journal (Refereed) Published
Abstract [en]

Colloidal quantum dots (QDs) have illuminated computer monitors and television screens due to their fascinating color-tunable properties depending on the size. Here, the electroluminescence (EL) wavelength of perovskite LEDs was tuned via the atomic layer number (ALN) of nanoplates (NPs) instead of the "size" in conventional QDs. We demonstrated efficient LEDs with controllably tailored emission from n = 3, 4, 5, and >= 7 ALN perovskite NPs with specific and discrete major peaks at 607, 638, 669, and 728 nanometers. These LEDs demonstrated peak external quantum efficiency (EQE) of 26.8% and high wavelength reproducibility with less than 1 to 2 nm difference between batches. High color stability without observable EL spectral change and operating stability with the best T50 of 267 minutes at 1.0 milliampere per square centimeter was also achieved. This work demonstrates a concept of tailoring specific ALN emission with fixed wavelengths, shedding light on efficient, emission-discrete, and color-stable LEDs for next-generation display.

Place, publisher, year, edition, pages
American Association for the Advancement of Science (AAAS) , 2025. Vol. 11, no 7, article id eadp9595
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Physical Sciences
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URN: urn:nbn:se:kth:diva-360817DOI: 10.1126/sciadv.adp9595ISI: 001421952400019PubMedID: 39951530Scopus ID: 2-s2.0-85218250132OAI: oai:DiVA.org:kth-360817DiVA, id: diva2:1941943
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QC 20250303

Available from: 2025-03-03 Created: 2025-03-03 Last updated: 2025-03-03Bibliographically approved

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Wang, Ligang

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