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Comparative measures of radionuclide containment in the crystalline geosphere
KTH, Superseded Departments (pre-2005), Land and Water Resources Engineering.ORCID iD: 0000-0002-5665-747x
Swedish Nuclear Fuel and Waste Management Company.ORCID iD: 0000-0001-9251-5367
2002 (English)In: Nuclear science and engineering, ISSN 0029-5639, E-ISSN 1943-748X, Vol. 142, no 3, p. 292-304Article in journal (Refereed) Published
Abstract [en]

A probabilistic model for assessing the capacity of a fractured crystalline rock volume to contain radionuclides is developed The rock volume is viewed as a network of discrete fractures through which radionuclides are transported by flowing water. Diffusive mass transfer between the open fractures and the stagnant water in the pore space of the rock matrix allow radionuclides access to mineral grains where physical and chemical processes-collectively known as sorption-can retain radionuclides. A stochastic Lagrangian framework is adopted to compute the probability that a radionuclide particle will be retained by the rock, i.e., the probability that it will decay before being released from the rock volume. A dimensionless quantity referred to as the containment index is related to this probability and proposed as a suitable measure for comparing different rock volumes; such a comparative measure may be needed, for example, in a site selection program for geological radioactive waste disposal. The probabilistic solution of the transport problem is based on the statistics of two Lagrangian variables: T, the travel time of an imaginary tracer moving with the flowing water, and beta, a suitably normalized surface area available for retention. Statistics of tau and beta may be computed numerically using site-specific discrete fracture MP network simulations. Fracture data from the well-characterized Aspo Hard Rock Laboratory site in southern Sweden are used to illustrate the implementation of the proposed containment index for six radionuclides (Sn-126, I-129, Cs-135, Np-237, Pu-239, and Se-79). It is found that fractures of small aperture imply prolonged travel times and hence long tails in both beta and tau. This, in turn, enhances retention and is favorable from a safely assessment perspective.

Place, publisher, year, edition, pages
Informa UK Limited , 2002. Vol. 142, no 3, p. 292-304
Keywords [en]
heterogeneous porous formations, granitic rock, fluid-flow, 3-dimensional networks, stochastic-analysis, matrix diffusion, solute transport, fractured media, mass-transport, model
National Category
Engineering and Technology
Identifiers
URN: urn:nbn:se:kth:diva-22038DOI: 10.13182/NSE02-A2308ISI: 000179173300004Scopus ID: 2-s2.0-0036862546OAI: oai:DiVA.org:kth-22038DiVA, id: diva2:340736
Note

QC 20230630

Available from: 2010-08-10 Created: 2010-08-10 Last updated: 2023-06-30Bibliographically approved

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Cvetkovic, VladimirSelroos, Jan-Olof

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