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Synthesis and application of chiral P,N-ligands with pseudo-meso and pseudo-C-2 symmetry
KTH, Tidigare Institutioner                               , Kemi.ORCID-id: 0000-0002-1743-7650
2001 (engelsk)Inngår i: Organic Letters, ISSN 1523-7060, E-ISSN 1523-7052, Vol. 3, nr 16, s. 2525-2528Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

[GRAPHICS] Two diastereoisomeric P,N-ligands, (S,S)-1 and (R,S)-1, were synthesized and assessed in palladium-catalyzed allylic alkylations. With rac-1,3-diphenylpropenyl acetate as substrate, ligand (AS)-1, with pseudo-C-2 symmetry, exhibited higher reactivity and higher enantioselectivity than the pseudo-meso ligand (R,S)-1, whereas reversal reactivity and selectivity were observed with rac-3-cyclohexenyl acetate.

sted, utgiver, år, opplag, sider
2001. Vol. 3, nr 16, s. 2525-2528
Emneord [en]
catalyzed allylic alkylation, bidentate ligands, substitutions, complexes, oxazolines
Identifikatorer
URN: urn:nbn:se:kth:diva-20864ISI: 000170392300027OAI: oai:DiVA.org:kth-20864DiVA, id: diva2:339561
Merknad
QC 20100525Tilgjengelig fra: 2010-08-10 Laget: 2010-08-10 Sist oppdatert: 2017-12-12bibliografisk kontrollert

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