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Testing tubewell platform color as a rapid screening tool for arsenic and manganese in drinking water wells
KTH, Skolan för arkitektur och samhällsbyggnad (ABE), Mark- och vattenteknik, Miljögeokemi och ekoteknik. (KTH-International Groundwater Arsenic Research Group)
KTH, Skolan för arkitektur och samhällsbyggnad (ABE), Mark- och vattenteknik, Miljögeokemi och ekoteknik. (KTH-International Groundwater Arsenic Research Group)ORCID-id: 0000-0003-4350-9950
KTH, Skolan för arkitektur och samhällsbyggnad (ABE), Mark- och vattenteknik, Miljögeokemi och ekoteknik. (KTH-International Groundwater Arsenic Research Group)
Vise andre og tillknytning
2012 (engelsk)Inngår i: Environmental Science and Technology, ISSN 0013-936X, E-ISSN 1520-5851, ISSN 0013-936X, Vol. 46, s. 434-440Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

A low-cost rapid screening tool for arsenic (As) and manganese (Mn) in groundwater is urgently needed to formulate mitigation policies for sustainable drinking water supply. This study attempts to make statistical comparison between tubewell (TW)platform color and the level of As and Mn concentration in groundwater extracted from the respective TW (n = 423), to validate platform color as a screening tool for As andMnin groundwater. The result shows that a black colored platform with 73% certainty indicates that well water is safe fromAs, while with 84% certainty a red colored platform indicates that well water is enriched with As, compared to WHO drinking waterguideline of 10 μg/L. With this guideline the efficiency, sensitivity, and specificity of the tool are 79%, 77%, and 81%, respectively.However, the certainty values become 93% and 38%, respectively, for black and redcolored platforms at 50 μg/L, the drinking water standards for India and Bangladesh. The respective efficiency, sensitivity, and specificity are 65%, 85%, and 59%. Similarly for Mn, black and red colored platform with 78% and 64% certainty, respectively, indicates that wellwater is either enriched or free from Mn at the Indian national drinking water standard of 300 μg/L. With this guideline the efficiency, sensitivity, and specificity of the tool are 71%, 67%, and 76%, respectively. Thus, this study demonstrates that TWplatform color can bepotentially used as an initial screening tool for identifying TWs with elevated dissolved As andMn, tomake further rigorous groundwater testing more intensive and implement mitigation options for safe drinking water supplies.

sted, utgiver, år, opplag, sider
American Chemical Society (ACS), 2012. Vol. 46, s. 434-440
HSV kategori
Identifikatorer
URN: urn:nbn:se:kth:diva-85973DOI: 10.1021/es203058aISI: 000298762900058Scopus ID: 2-s2.0-84855321319OAI: oai:DiVA.org:kth-85973DiVA, id: diva2:500337
Prosjekter
VR-Sida, Mistra, EURINDIA
Forskningsfinansiär
Swedish Research Council, 348-2006-6005
Merknad
QC 20120227Tilgjengelig fra: 2012-02-13 Laget: 2012-02-13 Sist oppdatert: 2017-12-07bibliografisk kontrollert
Inngår i avhandling
1. Arsenic Geochemistry in the Alluvial Aquifers of West Bengal, India: Implications for targeting safe aquifers for sustainable drinking water supply
Åpne denne publikasjonen i ny fane eller vindu >>Arsenic Geochemistry in the Alluvial Aquifers of West Bengal, India: Implications for targeting safe aquifers for sustainable drinking water supply
2013 (engelsk)Doktoravhandling, med artikler (Annet vitenskapelig)
Abstract [en]

The natural occurrences of high (>10 μg/L) dissolved arsenic (As) in groundwater of Bengal Basin has put millions of people under the threat of chronic As exposure through drinking water. Present study has examined the processes that regulate As mobilization and its distribution in shallow aquifers and the potentiality of finding safe aquifers within shallow depth (<50 m) for drinking water supply. The results indicate that in terms of aquifer sediment colors and water quality two types of aquifer namely brown sand aquifer (BSA) and grey sand aquifer (GSA) can be distinguished within the depth, accessible by low-cost drilling. The redox condition in the BSA is delineated to be Mn oxyhydroxides reducing, not sufficiently lowered for As mobilization resulting in high Mn and low Fe and As in groundwater. While in GSA, currently the reductive dissolution of Fe oxyhydroxides is the prevailing redox process causing As mobilization into groundwater of this aquifer type. It is revealed that the vertical distribution of As and other aqueous redox parameters is related to the redox zonation within aquifer. The decoupling of As and Fe release into groundwater is evident in the shallowest part of aquifer because of Fe enrichment by weathering of silicate minerals especially of biotite, the precipitation of secondary mineral phases like siderite and vivianite and incomplete reduction of Fe oxyhydroxides. It is characterized that the seasonal variations of As and other aqueous solutes are limited within the upper portion of aquifer only (<30 m bgl) and can be related to seasonal cycling of redox status, aggregation and dispersion of As scavenging colloids, local groundwater abstraction and monsoonal recharge. The results of surface complexation modeling indicate that PO43- is the major competitor of As(III) and As(V) adsorption onto Fe oxyhydroxides. This study concludes that the reductive dissolution of Fe oxyhydroxides followed by competitive sorption reactions with the aquifer sediment is the process conducive for As enrichment in groundwater of Bengal Basin. Present study advocates that despite low concentration of As in groundwater, a rigorous assessment of attendant health risk for Mn is necessary prior to considering mass scale exploitation of the BSA for sustainable drinking water supply. This study also validates that TW platform colors can be used as a rapid screening tool for As and Mn in drinking water wells to prioritize As mitigation management.

sted, utgiver, år, opplag, sider
Stockholm: KTH Royal Institute of Technology, 2013. s. xii, 71
Serie
TRITA-LWR. PHD, ISSN 1650-8602 ; 1071
Emneord
Bengal Basin; Groundwater; Arsenic; Redox processes; Competing ions; Sustainable drinking water Supply
HSV kategori
Identifikatorer
urn:nbn:se:kth:diva-128938 (URN)978-91-7501-849-2 (ISBN)
Disputas
2013-09-23, Kollegiesalen, Brinellvägen 8, KTH, Stockholm, 13:00 (engelsk)
Opponent
Veileder
Prosjekter
EURINDIA 2009-1665
Forskningsfinansiär
Mistra - The Swedish Foundation for Strategic Environmental Research, 2005-035-137
Merknad

QC 20130919

Tilgjengelig fra: 2013-09-19 Laget: 2013-09-17 Sist oppdatert: 2019-12-10bibliografisk kontrollert

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