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Testing tubewell platform color as a rapid screening tool for arsenic and manganese in drinking water wells
KTH, Skolan för arkitektur och samhällsbyggnad (ABE), Mark- och vattenteknik, Miljögeokemi och ekoteknik. (KTH-International Groundwater Arsenic Research Group)
KTH, Skolan för arkitektur och samhällsbyggnad (ABE), Mark- och vattenteknik, Miljögeokemi och ekoteknik. (KTH-International Groundwater Arsenic Research Group)ORCID-id: 0000-0003-4350-9950
KTH, Skolan för arkitektur och samhällsbyggnad (ABE), Mark- och vattenteknik, Miljögeokemi och ekoteknik. (KTH-International Groundwater Arsenic Research Group)
Visa övriga samt affilieringar
2012 (Engelska)Ingår i: Environmental Science and Technology, ISSN 0013-936X, E-ISSN 1520-5851, ISSN 0013-936X, Vol. 46, s. 434-440Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

A low-cost rapid screening tool for arsenic (As) and manganese (Mn) in groundwater is urgently needed to formulate mitigation policies for sustainable drinking water supply. This study attempts to make statistical comparison between tubewell (TW)platform color and the level of As and Mn concentration in groundwater extracted from the respective TW (n = 423), to validate platform color as a screening tool for As andMnin groundwater. The result shows that a black colored platform with 73% certainty indicates that well water is safe fromAs, while with 84% certainty a red colored platform indicates that well water is enriched with As, compared to WHO drinking waterguideline of 10 μg/L. With this guideline the efficiency, sensitivity, and specificity of the tool are 79%, 77%, and 81%, respectively.However, the certainty values become 93% and 38%, respectively, for black and redcolored platforms at 50 μg/L, the drinking water standards for India and Bangladesh. The respective efficiency, sensitivity, and specificity are 65%, 85%, and 59%. Similarly for Mn, black and red colored platform with 78% and 64% certainty, respectively, indicates that wellwater is either enriched or free from Mn at the Indian national drinking water standard of 300 μg/L. With this guideline the efficiency, sensitivity, and specificity of the tool are 71%, 67%, and 76%, respectively. Thus, this study demonstrates that TWplatform color can bepotentially used as an initial screening tool for identifying TWs with elevated dissolved As andMn, tomake further rigorous groundwater testing more intensive and implement mitigation options for safe drinking water supplies.

Ort, förlag, år, upplaga, sidor
American Chemical Society (ACS), 2012. Vol. 46, s. 434-440
Nationell ämneskategori
Naturvetenskap
Identifikatorer
URN: urn:nbn:se:kth:diva-85973DOI: 10.1021/es203058aISI: 000298762900058Scopus ID: 2-s2.0-84855321319OAI: oai:DiVA.org:kth-85973DiVA, id: diva2:500337
Projekt
VR-Sida, Mistra, EURINDIA
Forskningsfinansiär
Vetenskapsrådet, 348-2006-6005
Anmärkning
QC 20120227Tillgänglig från: 2012-02-13 Skapad: 2012-02-13 Senast uppdaterad: 2017-12-07Bibliografiskt granskad
Ingår i avhandling
1. Arsenic Geochemistry in the Alluvial Aquifers of West Bengal, India: Implications for targeting safe aquifers for sustainable drinking water supply
Öppna denna publikation i ny flik eller fönster >>Arsenic Geochemistry in the Alluvial Aquifers of West Bengal, India: Implications for targeting safe aquifers for sustainable drinking water supply
2013 (Engelska)Doktorsavhandling, sammanläggning (Övrigt vetenskapligt)
Abstract [en]

The natural occurrences of high (>10 μg/L) dissolved arsenic (As) in groundwater of Bengal Basin has put millions of people under the threat of chronic As exposure through drinking water. Present study has examined the processes that regulate As mobilization and its distribution in shallow aquifers and the potentiality of finding safe aquifers within shallow depth (<50 m) for drinking water supply. The results indicate that in terms of aquifer sediment colors and water quality two types of aquifer namely brown sand aquifer (BSA) and grey sand aquifer (GSA) can be distinguished within the depth, accessible by low-cost drilling. The redox condition in the BSA is delineated to be Mn oxyhydroxides reducing, not sufficiently lowered for As mobilization resulting in high Mn and low Fe and As in groundwater. While in GSA, currently the reductive dissolution of Fe oxyhydroxides is the prevailing redox process causing As mobilization into groundwater of this aquifer type. It is revealed that the vertical distribution of As and other aqueous redox parameters is related to the redox zonation within aquifer. The decoupling of As and Fe release into groundwater is evident in the shallowest part of aquifer because of Fe enrichment by weathering of silicate minerals especially of biotite, the precipitation of secondary mineral phases like siderite and vivianite and incomplete reduction of Fe oxyhydroxides. It is characterized that the seasonal variations of As and other aqueous solutes are limited within the upper portion of aquifer only (<30 m bgl) and can be related to seasonal cycling of redox status, aggregation and dispersion of As scavenging colloids, local groundwater abstraction and monsoonal recharge. The results of surface complexation modeling indicate that PO43- is the major competitor of As(III) and As(V) adsorption onto Fe oxyhydroxides. This study concludes that the reductive dissolution of Fe oxyhydroxides followed by competitive sorption reactions with the aquifer sediment is the process conducive for As enrichment in groundwater of Bengal Basin. Present study advocates that despite low concentration of As in groundwater, a rigorous assessment of attendant health risk for Mn is necessary prior to considering mass scale exploitation of the BSA for sustainable drinking water supply. This study also validates that TW platform colors can be used as a rapid screening tool for As and Mn in drinking water wells to prioritize As mitigation management.

Ort, förlag, år, upplaga, sidor
Stockholm: KTH Royal Institute of Technology, 2013. s. xii, 71
Serie
TRITA-LWR. PHD, ISSN 1650-8602 ; 1071
Nyckelord
Bengal Basin; Groundwater; Arsenic; Redox processes; Competing ions; Sustainable drinking water Supply
Nationell ämneskategori
Geovetenskap och miljövetenskap
Identifikatorer
urn:nbn:se:kth:diva-128938 (URN)978-91-7501-849-2 (ISBN)
Disputation
2013-09-23, Kollegiesalen, Brinellvägen 8, KTH, Stockholm, 13:00 (Engelska)
Opponent
Handledare
Projekt
EURINDIA 2009-1665
Forskningsfinansiär
Mistra - Stiftelsen för miljöstrategisk forskning, 2005-035-137
Anmärkning

QC 20130919

Tillgänglig från: 2013-09-19 Skapad: 2013-09-17 Senast uppdaterad: 2019-12-10Bibliografiskt granskad

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Förlagets fulltextScopushttp://pubs.acs.org/doi/abs/10.1021/es203058a

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