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Walnut shells as a potential low-cost lignocellulosic sorbent for dyes and metal ions
Igor Sikorsky Kyiv Polytech Inst, Fac Chem Engn, Dept Ecol & Technol Plant Polymers, Peremogy Avenu 37-4, UA-03056 Kiev, Ukraine.;Natl Acad Sci Ukraine, OO Chuiko Inst Surface Chem, Gen Naumov Str 17, UA-03164 Kiev, Ukraine..
KTH, Skolan för kemi, bioteknologi och hälsa (CBH), Fiber- och polymerteknologi. KTH, Skolan för kemi, bioteknologi och hälsa (CBH), Centra, Wallenberg Wood Science Center.
KTH, Skolan för kemi, bioteknologi och hälsa (CBH), Fiber- och polymerteknologi. KTH, Skolan för kemi, bioteknologi och hälsa (CBH), Centra, Wallenberg Wood Science Center.
Kyiv Natl Univ Trade & Econ, Kyoto Str 19, UA-02156 Kiev, Ukraine..
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2018 (Engelska)Ingår i: Cellulose (London), ISSN 0969-0239, E-ISSN 1572-882X, Vol. 25, nr 8, s. 4729-4742Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

Currently, it is necessary to develop new methods and materials for solving the problem of environmental pollution by various toxicants. For these purposes, vegetal materials can be used. In this study, efficient low-cost sorbents based on walnut shells, an agro-industrial by-product, were prepared by treatment with acetic acid or a mixture of acetic acid and hydrogen peroxide. It was shown that the treatments significantly affected the composition and structure of walnut shells and their sorption properties with respect to organic dyes (methylene blue, methyl violet, and murexide) and heavy metal ions. Methylene blue dye was used for additional studies on the effect of pH, contact time and kinetics of sorption. The maximum adsorption rate of the dye occurred within the first 30 min of contact, during which the concentration of methylene blue in the solution was reduced by more than half. Full sorption equilibrium was reached within 180-230 min for studied samples. The adsorption kinetics of methylene blue was found to best be described by pseudo-second-order kinetic model. It was shown that dyes adsorption processes were well described by Freundlich model, which takes into consideration the heterogeneity of the surface of the adsorbent. The obtained plant sorbents are characterized by a high sorption capacity for heavy metal ions (18-29 mg/g for Fe3+ and 33-44 mg/g for Cu-2). Due to their numerous advantages, such as the high sorption capacity, high availability and low cost of raw materials, simplicity of disposal and nontoxicity, the obtained natural sorbents may have a wide practical use in industrial wastewater treatment. [GRAPHICS] .

Ort, förlag, år, upplaga, sidor
Springer, 2018. Vol. 25, nr 8, s. 4729-4742
Nyckelord [en]
Walnut shells, Cellulose, Lignin, Dye, Metals, Sorption
Nationell ämneskategori
Polymerteknologi
Identifikatorer
URN: urn:nbn:se:kth:diva-232598DOI: 10.1007/s10570-018-1896-yISI: 000438276000032Scopus ID: 2-s2.0-85048377766OAI: oai:DiVA.org:kth-232598DiVA, id: diva2:1236131
Anmärkning

QC 20180731

Tillgänglig från: 2018-07-31 Skapad: 2018-07-31 Senast uppdaterad: 2019-05-02Bibliografiskt granskad

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Sevastyanova, OlenaLindström, Mikael

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Sevastyanova, OlenaRiazanova, Anastasia V.Budnyak, TetyanaLindström, Mikael
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Fiber- och polymerteknologiWallenberg Wood Science Center
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Cellulose (London)
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