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Multidimensional resonant nonlinear spectroscopy with coherent broadband x-ray pulses
Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.;Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA..
Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA..
Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA..ORCID-id: 0000-0002-2288-2548
KTH, Skolan för bioteknologi (BIO), Teoretisk kemi och biologi. Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.;KTH Royal Inst Technol, Sch Biotechnol, Dept Theoret Chem & Biol, S-10691 Stockholm, Sweden..ORCID-id: 0000-0002-6706-651X
Vise andre og tillknytning
2016 (engelsk)Inngår i: Physica Scripta, ISSN 0031-8949, E-ISSN 1402-4896, Vol. T169, artikkel-id 014002Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

New x-ray free electron laser (XFEL) and high harmonic generation (HHG) light sources are capable of generating short and intense pulses that make x-ray nonlinear spectroscopy possible. Multidimensional spectroscopic techniques, which have long been used in the nuclear magnetic resonance, infrared, and optical regimes to probe the electronic structure and nuclear dynamics of molecules by sequences of short pulses with variable delays, can thus be extended to the attosecond x-ray regime. This opens up the possibility of probing core-electronic structure and couplings, the real-time tracking of impulsively created valence-electronic wavepackets and electronic coherences, and monitoring ultrafast processes such as nonadiabatic electron-nuclear dynamics near conical-intersection crossings. We survey various possible types of multidimensional x-ray spectroscopy techniques and demonstrate the novel information they can provide about molecules.

sted, utgiver, år, opplag, sider
IOP PUBLISHING LTD , 2016. Vol. T169, artikkel-id 014002
Emneord [en]
x-ray, spectroscopy, Raman, four-wave-mixing
HSV kategori
Identifikatorer
URN: urn:nbn:se:kth:diva-242662DOI: 10.1088/0031-8949/T169/1/014002ISI: 000413519600002Scopus ID: 2-s2.0-85021180184OAI: oai:DiVA.org:kth-242662DiVA, id: diva2:1291360
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QC 20190225

Tilgjengelig fra: 2019-02-25 Laget: 2019-02-25 Sist oppdatert: 2019-02-25bibliografisk kontrollert

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Hua, Weijie

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