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The Use of Layer-by-Layer Self-Assembly and Nanocellulose to Prepare Advanced Functional Materials
KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Fibre- and Polymer Technology, Fibre Technology. KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Centres, Wallenberg Wood Science Center.ORCID iD: 0000-0001-8622-0386
KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Fibre- and Polymer Technology, Fibre Technology.ORCID iD: 0000-0003-1874-2187
2021 (English)In: Advanced Materials, ISSN 0935-9648, E-ISSN 1521-4095, Vol. 33, no 28, article id 2001474Article, review/survey (Refereed) Published
Abstract [en]

The current knowledge about the formation of layer-by-layer (LbL) self-assemblies using combinations of nanocelluloses (NCs) and polyelectrolytes is reviewed. Herein, the fundamentals behind the LbL formation, with a major focus on NCs, are considered. Following this, a special description of the limiting factors for the formation of LbLs of only NCs, both anionic and cationic, and the combination of NCs and polyelectrolytes/nanoparticles is provided. The ability of the NCs and polyelectrolytes to form dense films with excellent mechanical properties and with tailored optical properties is then reviewed. How low-density, wet stable networks of cellulose nanofibrils can be used as substrates for the preparation of antibacterial, electrically interactive, and fire-retardant materials by forming well-defined LbLs inside these networks is then considered. A short outlook of the possible uses of LbLs containing NCs is given to conclude.

Place, publisher, year, edition, pages
Wiley , 2021. Vol. 33, no 28, article id 2001474
Keywords [en]
cellulose nanocrystals, cellulose nanofibrils, layer-by-layer structures, polyelectrolytes
National Category
Paper, Pulp and Fiber Technology
Identifiers
URN: urn:nbn:se:kth:diva-303486DOI: 10.1002/adma.202001474ISI: 000556252500001PubMedID: 32767441Scopus ID: 2-s2.0-85089076696OAI: oai:DiVA.org:kth-303486DiVA, id: diva2:1603171
Note

QC 20211014

Available from: 2021-10-14 Created: 2021-10-14 Last updated: 2022-06-25Bibliographically approved

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Wågberg, LarsErlandsson, Johan

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