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Photon Up-Conversion via Epitaxial Surface-Supported Metal-Organic Framework Thin Films with Enhanced Photocurrent
Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China..
Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China..
Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China..
Dalian Univ Technol, Inst Artificial Photosynth, State Key Lab Fine Chem, Dalian 116024, Peoples R China..ORCID iD: 0000-0002-5405-6398
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2018 (English)In: ACS Applied Energy Materials, E-ISSN 2574-0962, Vol. 1, no 2, p. 249-253Article in journal (Refereed) Published
Abstract [en]

We report a new triplet-triplet annihilation photon up-conversion (TTA-UC) system using an epitaxial Zn-perylene surface-supported metal-organic framework (SURMOF) grown on metal oxide surface as "emitter", and a platinum octaethylporphyrin (PtOEP) as "sensitizer" in [Co(bpy)(3)](2+/3+) acetonitrile solution. It has been demonstrated that the photocurrent can be significantly enhanced relative to epitaxial Zn-perylene SURMOF due to the TTA-UC mechanism. This initial result holds promising applications toward SURMOF-based solar energy conversion devices.

Place, publisher, year, edition, pages
American Chemical Society (ACS) , 2018. Vol. 1, no 2, p. 249-253
Keywords [en]
triplet-triplet annihilation, up-conversion, metal-organic framework thin film, photocurrent
National Category
Physical Chemistry
Identifiers
URN: urn:nbn:se:kth:diva-303832DOI: 10.1021/acsaem.7b00023ISI: 000458705100003Scopus ID: 2-s2.0-85051468004OAI: oai:DiVA.org:kth-303832DiVA, id: diva2:1605203
Note

QC 20211022

Available from: 2021-10-22 Created: 2021-10-22 Last updated: 2022-06-25Bibliographically approved

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Sun, Licheng

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