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Influence of the magnetic sublattices in the double perovskite LaCaNiReO6
Chalmers Univ Technol, Dept Phys, S-41296 Gothenburg, Sweden..
KTH, School of Engineering Sciences (SCI), Applied Physics, Materials and Nanophysics. Chalmers Univ Technol, Dept Phys, S-41296 Gothenburg, Sweden..ORCID iD: 0000-0001-8879-7875
KTH, School of Engineering Sciences (SCI), Applied Physics, Materials and Nanophysics.ORCID iD: 0000-0003-4441-8882
KTH, School of Engineering Sciences (SCI), Applied Physics. Uppsala Univ, Div Mol & Condensed Matter Phys, S-75237 Uppsala, Sweden.;Sorbonne Univ, Inst Nanosci Paris, UMR CNRS 7588, F-75005 Paris, France..ORCID iD: 0000-0002-6471-1093
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2022 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 106, no 21, article id 214410Article in journal (Refereed) Published
Abstract [en]

The magnetism of double perovskites is a complex phenomenon, determined from intra- or interatomic magnetic moment interactions, and strongly influenced by geometry. We take advantage of the complementary length and timescales of the muon spin rotation, relaxation, and resonance (mu+SR) microscopic technique and bulk ac/dc magnetic susceptibility measurements to study the magnetic phases of the LaCaNiReO6 double perovskite. As a result, we are able to discern and report ferrimagnetic ordering below TC = 102 K and the formation of different magnetic domains above TC. Between TC < T < 270 K, the following two magnetic environments appear, a dense spin region and a static-dilute spin region. The paramagnetic state is obtained only above T > 270 K. An evolution of the interaction between Ni and Re magnetic sublattices, in this geometrically frustrated fcc perovskite structure, is revealed as a function of temperature through the critical behavior and thermal evolution of microscopic and macroscopic physical quantities.

Place, publisher, year, edition, pages
American Physical Society (APS) , 2022. Vol. 106, no 21, article id 214410
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Condensed Matter Physics
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URN: urn:nbn:se:kth:diva-323353DOI: 10.1103/PhysRevB.106.214410ISI: 000901993200003Scopus ID: 2-s2.0-85143683804OAI: oai:DiVA.org:kth-323353DiVA, id: diva2:1731495
Note

QC 20230127

Available from: 2023-01-27 Created: 2023-01-27 Last updated: 2023-12-07Bibliographically approved

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Forslund, Ola KenjiNocerino, ElisabettaJohansson, FredrikMatsubara, NamiMånsson, Martin

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