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An insight into the protonation property of a diiron azadithiolate complex pertinent to the active site of Fe-only hydirogenases
Vise andre og tillknytning
2006 (engelsk)Inngår i: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, nr 3, s. 305-307Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

Protonation of [{(mu-SCH2)(2)N(C6H4-p-NO2)}{Fe(CO)(2)(PMe3)}(2)] in the presence of 4 equiv. of HOTf afforded two species, a mu-hydride diiron complex, the molecular structure of which was crystallographically characterized, and a p-S-protonated species, which was readily deprotonated in the presence of pyridine.

sted, utgiver, år, opplag, sider
2006. nr 3, s. 305-307
Emneord [en]
density-functional calculations, model complexes, hydrogen evolution, bridging ligand, iron, mimics, activation, dihydrogen, mechanism, h-2
Identifikatorer
URN: urn:nbn:se:kth:diva-15404DOI: 10.1039/b513270cISI: 000235034700035Scopus ID: 2-s2.0-33645461565OAI: oai:DiVA.org:kth-15404DiVA, id: diva2:333445
Merknad
QC 20100525Tilgjengelig fra: 2010-08-05 Laget: 2010-08-05 Sist oppdatert: 2017-12-12bibliografisk kontrollert

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