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Electro-optic effect in ferroelectric Na0.5K0.5NbO3 thin films on oxide substrates
KTH, Skolan för informations- och kommunikationsteknik (ICT), Mikroelektronik och Informationsteknik, IMIT.
KTH, Skolan för informations- och kommunikationsteknik (ICT), Materialfysik, Materialfysik, MF.ORCID-id: 0000-0001-8774-9302
KTH, Skolan för informations- och kommunikationsteknik (ICT), Mikroelektronik och Informationsteknik, IMIT.
2006 (Engelska)Ingår i: Integrated Ferroelectrics, ISSN 1058-4587, E-ISSN 1607-8489, Vol. 80, nr 1, s. 97-106Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

We have deposited Na0.5NbO3 (NKN) films oil single crystal Al2O3(1 (1) under bar 02) and SrTiO3(001) substrates using rf-magnetron sputtering of a stoichiometric, high-density ceramic target. Using x-ray diffraction it was confirmed that NKN grows preferentially c-axis oriented on sapphire substrate and epitaxially oil the perovskite SrTiO3(001) substrate. Electro-optical (EO) properties were measured in visible light through a transverse method. With an applied dc field up to 20 kV/cm, the effective linear EO response was determined to r(eff) = 28 pm/V for NKN/Al2O3 and r(eff) = I I pm/V for NKN/SrTiO3, where a superlinear dependence was observed.

Ort, förlag, år, upplaga, sidor
2006. Vol. 80, nr 1, s. 97-106
Nyckelord [en]
sodium potassium mobates, ferroelectric films, rf-rnagnetron sputtering, XRD, electro-optic effects, AFM, pulsed-laser deposition, knbo3
Nationell ämneskategori
Annan materialteknik
Identifikatorer
URN: urn:nbn:se:kth:diva-15800DOI: 10.1080/10584580600656569ISI: 000238680700012Scopus ID: 2-s2.0-33745751799OAI: oai:DiVA.org:kth-15800DiVA, id: diva2:333842
Anmärkning
QC 20100525, QC 20110929. Conference: 17th International Symposium on Integrated Ferroelectrics .Shanghai, PEOPLES R CHINA. APR 17-20, 2005 Tillgänglig från: 2010-08-05 Skapad: 2010-08-05 Senast uppdaterad: 2017-12-12Bibliografiskt granskad
Ingår i avhandling
1. Electro-Optical Na0.5K0.5NbO3 Films
Öppna denna publikation i ny flik eller fönster >>Electro-Optical Na0.5K0.5NbO3 Films
2005 (Engelska)Doktorsavhandling, sammanläggning (Övrigt vetenskapligt)
Abstract [en]

Ferroelectric oxides are a group of advanced electronic materials with a wide variety of properties useful in applications such as memory devices, resonators and filters, infrared sensors, microelectromechanical systems, and optical waveguides and modulators.

Among the oxide perovskite-structured ferroelectric thin film materials, sodium potassium niobate or Na0.5K0.5NbO3 (NKN) has recently emerged as one of the most promising materials in radio frequency (rf) and microwave applications due to high dielectric tenability and low dielectric loss.

This thesis presents results on growth and structural, optical, and electrical characterization of NKN thin films. The films were deposited by rf-magnetron sputtering of a stoichiometric, high density, ceramic Na0.5K0.5NbO3 target onto single crystal LaAlO3 (LAO), Al2O3 (sapphire), SrTiO3, and Nd:YAlO3, and polycrystalline Pt80Ir20 substrates. By x-ray diffractometry, NKN films on c-axis oriented LaAlO3, SrTiO3 and Nd:YAlO3 substrates were found to grow epitaxially, whereas films on r-cut sapphire and polycrystalline Pt80Ir20 substrates were found to be preferentially (00l) oriented. The surface morphology was explored using atomic force microscopy.

Optical and waveguiding properties of the Na0.5K0.5NbO3/substrate heterostructures were characterized using prism-coupling technique. Sharp and distinguishable transverse magnetic and electric propagation modes were observed for NKN thicknesses up to 2.0 μm. The extraordinary and ordinary refractive indices were calculated together with the birefringence of the NKN material. The electro-optic effect in transverse geometry was measured in transmission, where the effective linear electro-optic response was determined to reff = 28 pm/V for NKN/Al2O3 with an applied dc field up to 18 kV/cm.

The ferroelectric state in NKN films on Pt80Ir20 at room temperature was indicated by a polarization loop with saturated polarization as high as 33.4 μC/cm2 at 700 kV/cm, remnant polarization of 10 μC/cm2, and coercive field of 90 kV/cm. Current-voltage characteristics of vertical Au/NKN/PtIr capacitive cells and planar Au/NKN/LAO interdigital capacitors (IDCs) showed very good insulating properties, with the leakage current density for an NKN IDC on the order of 30 nA/cm2 at 400 kV/cm. Rf dielectric spectroscopy demonstrated low loss, low frequency dispersion, and high voltage tunability. At 1 MHz, NKN/LAO showed a dissipation factor tan δ = 0.010 and a tunability of 16.5 % at 200 kV/cm. For the same structure the frequency dispersion was Δεr = 8.5 % between 1 kHz and 1 MHz.

Ort, förlag, år, upplaga, sidor
Stockholm: KTH, 2005. s. xii, 91
Serie
Trita-FYS, ISSN 0280-316X ; 5299
Nyckelord
Functional materials, ferroelectrics, sodium potassium niobates, thin films, rf-magnetron sputtering, waveguiding, refractive index, prism-coupling, electro-optic effects, dielectric tunability, Funktionella material
Nationell ämneskategori
Annan materialteknik
Identifikatorer
urn:nbn:se:kth:diva-193 (URN)91-7178-007-6 (ISBN)
Disputation
2005-05-20, D1, KTH, Lindstedtsvägen 17, 2tr, Stockholm, 10:00
Opponent
Handledare
Anmärkning
QC 20100928Tillgänglig från: 2005-05-12 Skapad: 2005-05-12 Senast uppdaterad: 2010-09-28Bibliografiskt granskad

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Khartsev, Sergiy

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Blomqvist, MatsKhartsev, SergiyGrishin, Alexander M.
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Integrated Ferroelectrics
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