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Atmospheric water droplets can catalyse atom pair break-up via surface-induced resonance repulsion
KTH, Skolan för industriell teknik och management (ITM), Materialvetenskap, Flerskalig materialmodellering.
KTH, Skolan för industriell teknik och management (ITM), Materialvetenskap, Flerskalig materialmodellering.ORCID-id: 0000-0002-9050-5445
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2013 (engelsk)Inngår i: Europhysics letters, ISSN 0295-5075, E-ISSN 1286-4854, Vol. 101, nr 4, s. 43002-Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

We present the theory for a retarded resonance interaction between two identical atoms near a dielectric surface. In free space the resonance interaction between isotropically excited atom pairs is attractive at all atom-atom separations. We illustrate numerically how this interaction between oxygen, sulphur, hydrogen, or nitrogen atom pairs may turn repulsive near water droplets. The results provide evidence of a mechanism causing excited state atom pair breakage to occur in the atmosphere near water droplets.

sted, utgiver, år, opplag, sider
2013. Vol. 101, nr 4, s. 43002-
Emneord [en]
Correlated Molecular Calculations, Dipole-Dipole Interaction, Gaussian-Basis Sets, Microcavity, Energy
HSV kategori
Identifikatorer
URN: urn:nbn:se:kth:diva-120314DOI: 10.1209/0295-5075/101/43002ISI: 000315999100007Scopus ID: 2-s2.0-84874905845OAI: oai:DiVA.org:kth-120314DiVA, id: diva2:614298
Forskningsfinansiär
Swedish Research Council, C0485101 70529001
Merknad

QC 20130404

Tilgjengelig fra: 2013-04-04 Laget: 2013-04-04 Sist oppdatert: 2017-12-06bibliografisk kontrollert

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