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Fluorescence dynamics and rate equations analysis in Er3+,Yb3+ doped double tungstates
KTH, Skolan för teknikvetenskap (SCI), Tillämpad fysik, Laserfysik.
KTH, Skolan för teknikvetenskap (SCI), Tillämpad fysik, Laserfysik.
KTH, Skolan för teknikvetenskap (SCI), Tillämpad fysik, Laserfysik.ORCID-id: 0000-0002-2508-391X
Fisica I Cristal-Lografia de Materials (FiCMA), Universitat Rovira I Virgili, Spain.
Vise andre og tillknytning
2006 (engelsk)Inngår i: Applied Optics, ISSN 1559-128X, E-ISSN 2155-3165, Vol. 45, nr 19, s. 4715-4725Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

The fluorescence dynamics in Er3+ and Yb3+ doped KGd(WO4)(2) and KY(WO4)(2) has been investigated. Lifetimes have been measured for the Yb(F-2(5/2)), Er(I-4(13/2)), and Er(S-4(3/2)) levels around 1, 1.5, and 0.55 mu m, respectively. The Yb(F-2(5/2)) lifetimes show a decreasing trend toward the limiting Er(I-4(11/2)) lifetime with increasing Er-to-Yb concentration ratio, whereas the Er(I-4(13/2)) lifetimes are mostly unaffected by the doping concentrations. A rate equation analysis has been performed to explain the observed behavior and gain is calculated for a continuous-wave laser at 1.53 mu m to find the optimum doping concentrations for high gain.

sted, utgiver, år, opplag, sider
2006. Vol. 45, nr 19, s. 4715-4725
Emneord [en]
Continuous-wave lasers; Doping concentrations; Fluorescence dynamics; Rate equation analysis; Concentration (process); Equations of state of solids; Erbium compounds; Semiconductor doping; Solid state lasers; Tungsten compounds; Ytterbium compounds
HSV kategori
Identifikatorer
URN: urn:nbn:se:kth:diva-5454DOI: 10.1364/AO.45.004715ISI: 000238665900028Scopus ID: 2-s2.0-33746174995OAI: oai:DiVA.org:kth-5454DiVA, id: diva2:9824
Merknad
QC 20100713. Uppdaterad från Accepted till Published 20100713.Tilgjengelig fra: 2006-03-13 Laget: 2006-03-13 Sist oppdatert: 2017-11-21bibliografisk kontrollert
Inngår i avhandling
1. Diode-pumped rare-earth-doped quasi-three-level lasers
Åpne denne publikasjonen i ny fane eller vindu >>Diode-pumped rare-earth-doped quasi-three-level lasers
2005 (engelsk)Doktoravhandling, med artikler (Annet vitenskapelig)
Abstract [en]

Many rare-earth-doped materials are suitable for laser operation and this thesis focuses on diode-pumped solid-state lasers employing crystals doped with the trivalent rare-earth ions neodymium (Nd3+), ytterbium (Yb3+) and erbium (Er3+). Especially, the quasi-three-level transitions in Nd and Yb have been studied as well as the eye-safe three-level transition around 1.5 µm in Er.

Quasi-three-level laser transitions in neodymium-doped crystals such as Nd:YAG, Nd:YLF and Nd:YVO4 have received a great deal of interest because they allow for generation of blue light by frequency doubling. For solid-state blue laser sources, there exist numerous applications as in high-density optical data storage, colour displays, submarine communication and biological applications.

Efficient lasing on quasi-three-level transitions at 900¬–950 nm in Nd-doped crystals is considerably more difficult to achieve than on the stronger four-level transitions at 1–1.1 µm. The problems with these quasi-three-level transitions are a significant reabsorption loss at room temperature and a small stimulated emission cross section. This requires a tight focusing of the pump light, which is achieved by end-pumping with high-intensity diode lasers. Nd:YAG lasers at the 946 nm transition have been built and a maximum power of 7.0 W was obtained. By inserting a thin quartz etalon in the laser cavity, the 938.5 nm laser line could be selected and an output power of 3.9 W was then obtained.

By using nonlinear crystals, frequency-doubling of laser light at both 946 nm and 938.5 nm was achieved. Efficient generation of blue light at 473 nm has been obtained in periodically poled KTP, both in single-pass extra-cavity and intracavity configurations. More than 0.5 W was obtained at 473 nm by intracavity doubling. Intracavity second harmonic generation of the 938.5 nm transition gave slightly more than 200 mW at 469 nm.

During recent years, Yb-doped double-tungstate crystals like KGW and KYW have shown efficient laser operation. A comparative, experimental study of the laser performance and thermal-lensing properties between standard b-cut Yb:KGW and Yb:KGW cut along a novel athermal direction is presented. The results show that the thermal lens is about two times weaker and less astigmatic in the athermal-direction-cut crystal, for the same absorbed power. Also, Er-Yb-doped KGW and KYW have been investigated and the fluorescence dynamics have been measured for the Yb (2F5/2), Er (4I13/2) and Er (4S3/2) levels around 1 µm, 1.5 µm and 0.55 µm, respectively.

The influence of upconversion is a detrimental effect both in Nd-doped and Er-Yb-doped lasers. Analytical models starting from rate equations have been developed for these lasers including the influence of upconversion effects. The results of the general models have been applied to 946 nm Nd:YAG lasers and to Er-Yb-doped double-tungstate crystals in order to find the optimum doping concentrations for high gain for an eye-safe laser at 1.53 µm.

sted, utgiver, år, opplag, sider
Stockholm: KTH, 2005. s. viii, 86
Serie
Trita-FYS, ISSN 0280-316X ; 2005:70
Emneord
Optics, laser optics
HSV kategori
Identifikatorer
urn:nbn:se:kth:diva-544 (URN)91-7178-220-6 (ISBN)
Disputas
2005-12-16, Sal FD5, AlbaNova, Roslagstullsbacken 21, Stockholm, 10:00 (engelsk)
Opponent
Veileder
Merknad
QC 20100901Tilgjengelig fra: 2005-12-08 Laget: 2005-12-08 Sist oppdatert: 2010-09-01bibliografisk kontrollert
2. Novel materials for Yb and Er-Yb doped microchip lasers
Åpne denne publikasjonen i ny fane eller vindu >>Novel materials for Yb and Er-Yb doped microchip lasers
2006 (engelsk)Licentiatavhandling, med artikler (Annet vitenskapelig)
Abstract [en]

The objective of this thesis has been to investigate novel host material configurations for high-power end-pumped Er-Yb co-doped, or Yb doped microchip lasers and try to increase their performance. In Er-Yb co-doped systems, the main limitation is the thermal shortcomings of the phosphate glass host material. The thesis presents some novel results that contribute to the search for a crystalline replacement. In Yb doped systems, most end-pumped schemes reported have been using relatively low-power single-emitter diodes. The thesis presents experiments with Yb:KGW microchips end-pumped by high-power diode bars. Another common limitation of end-pumped Yb microchip lasers is the thermal lens that destabilizes the cavity and decreases the beam quality. The approach to reduce the thermal lens by using an athermal propagation direction has been evaluated and the results are presented in the thesis.

In the search for a crystalline host material for Er-Yb systems, borates have been found increasingly interesting. Consequently, we started out by investigating Gadolinium-calcium-oxoborate, GdCOB, which could be grown in platinum crucibles. It was found that the cw performance of such monolithic microchips is quite comparable to glass hosts in terms of slope efficiency, but the threshold is significantly larger. As for Q-switched performance, which is essential to most Er-Yb applications, the first efficient Q-switched results with a crystalline host is presented in the thesis. Similar to the cw regime, the slope efficiencies are comparable to glass, while the threshold is quite high. However, the perhaps most important parameter, maximum output power before thermal fracture, is neither significantly improved nor worsened compared with phosphate glass. This is believed to be due to higher threshold and a stronger thermal expansion that negates the benefit of a thermal conductivity that is only 2-3 times higher. To find a host material that could withstand higher pump powers, we turned our attention to the double-tungstates KGW and KYW, which have higher thermal conductivity and higher cross-sections. They have, however, energy level lifetimes which differ significantly from glass or borates and as a consequence, a thorough spectroscopic investigation has been undertaken to optimize dopant concentrations. Laser experiments on crystals with dopant concentrations based on this investigation are expected in the near future.

When pumping Yb:KGW with a high-power diode bar, we achieved output powers of 9 – 12.4 W under different experimental conditions with incident powers of 18.3 – 26 W. The incident power of 26 W in one design was enough to fracture the crystal. Using a crystal cut for propagation along an athermal direction and comparing it with an identical b-cut crystal, we found that the thermal lens in the athermally oriented crystal was about a factor two weaker at the same absorbed power.

sted, utgiver, år, opplag, sider
Stockholm: KTH, 2006. s. vii, 56
Serie
Trita-FYS, ISSN 0280-316X ; 2006:19
Emneord
mid-IR lasers, laser materials
HSV kategori
Identifikatorer
urn:nbn:se:kth:diva-3874 (URN)91-7178-299-0 (ISBN)
Presentation
2006-03-31, FA31, AlbaNova, Roslagstullsbacken 21, STOCKHOLM, 13:00
Opponent
Veileder
Merknad
QC 20101116Tilgjengelig fra: 2006-03-13 Laget: 2006-03-13 Sist oppdatert: 2010-11-16bibliografisk kontrollert
3. On diode-pumped solid-state lasers
Åpne denne publikasjonen i ny fane eller vindu >>On diode-pumped solid-state lasers
2007 (engelsk)Doktoravhandling, med artikler (Annet vitenskapelig)
Abstract [en]

The research that is presented in this thesis can be divided into two major parts. The first part concerns longitudinally pumped, bulk Er-Yb lasers. In these lasers, the main limitation is the thermal shortcomings of the phosphate glass host material. From the laser experiments and the spectroscopic measurements on crystalline host materials, as well as an investigation to bring further light to the physical background of the involved dynamics, the thesis presents some novel results that contribute to the search for a crystalline replacement. The second part concerns novel laser concepts applied to Yb-doped double tungstate lasers. Different crystal orientations are investigated, such as an athermal orientation for reduced thermal lensing and a conical refraction orientation for complete polarization tuning. Furthermore, the introduction of volume Bragg gratings in the cavity enables wide spectral tuning ranges and extremely low quantum defects.

Regarding the first part, the main results are the achievement of 15 % slope efficiency in a monolithic, continuous-wave Yb:GdCOB laser and the achievement of Q-switching of the same laser. The Q-switched pulse durations were around 5-6 ns and the Q-switched slope efficiency was 11.6 %. For both lasers, a maximum output power of 90 mW was obtained, which is close to ordinary glass lasers under similar conditions. A spectroscopic investigation into the Er,Yb-codoped double tungstates was also performed and the results have enabled mathematical modeling of the fluorescence dynamics in these materials. Finally, the temperature dependence of the dynamics in Er,Yb:YAG was studied and the results have given some insight into the physical background of the mechanisms involved.

Regarding the second part, different end-pumped Yb:KReW laser cavities were constructed to demonstrate the different concepts. With a laser crystal cut for propagation along the athermal direction at 17º angle clockwise from the dielectric direction Nm, the thermal lens could be reduced by 50 %. In these experiments the maximum output power was 4 W at 60 % slope efficiency. In another cavity incorporating a volume Bragg grating in a retroreflector set-up, the wavelength could be continuously tuned between 997 - 1050 nm. The spectral bandwidth was 10 GHz and the peak output power was 3 W. The same output power could also be obtained at 1063 nm with the grating positioned as an output coupler instead. If, on the other hand, the grating was positioned as an input coupler, 3.6 W output power at 998 nm was obtained at a quantum defect of only 1.6 %. Furthermore, using a crystal oriented for propagation along an optic axis, internal conical refraction could be used to establish arbitrary control of the polarization direction as well as the extinction ratio. Even unpolarized light could be enforced despite the highly anisotropic medium. With this configuration, the maximum output power was 8.6 W at 60 % slope efficiency which equals the performance of a reference crystal with standard orientation. The completely novel concepts of laser tuning with Bragg grating retroreflectors, of low quantum defect through Bragg grating input couplers and of polarization tuning by internal conical refraction can all easily be applied to several other laser materials as well.

sted, utgiver, år, opplag, sider
Stockholm: KTH, 2007. s. 76
Serie
Trita-FYS, ISSN 0280-316X ; 2007:81
Emneord
near-infrared lasers, end-pumped lasers, Q-switching, erbium, ytterbium, GdCOB, KGW, KYW, Co:MALO, laser materials, thermal lensing, end-pumping, spectroscopy, conical refraction, volume Bragg gratings, holographic gratings, laser tuning
HSV kategori
Identifikatorer
urn:nbn:se:kth:diva-4580 (URN)978-91-7178-841-2 (ISBN)
Disputas
2008-01-18, FA32, AlbaNova, Roslagstullsbacken 21, Stockholm, 10:00
Opponent
Veileder
Merknad
QC 20100713Tilgjengelig fra: 2007-12-14 Laget: 2007-12-14 Sist oppdatert: 2010-07-14bibliografisk kontrollert

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