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Stimulated X-ray Raman scattering: a critical assessment of the building block of nonlinear X-ray spectroscopy
KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.ORCID iD: 0000-0003-1269-8760
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2016 (English)In: Faraday discussions (Online), ISSN 1359-6640, E-ISSN 1364-5498Article in journal (Refereed) Published
Abstract [en]

With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets.

Place, publisher, year, edition, pages
Royal Society of Chemistry, 2016.
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Atom and Molecular Physics and Optics
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URN: urn:nbn:se:kth:diva-194073DOI: 10.1039/C6FD00103CISI: 000392422200014Scopus ID: 2-s2.0-85007500674OAI: oai:DiVA.org:kth-194073DiVA: diva2:1037215
Note

QC 20161017

Available from: 2016-10-14 Created: 2016-10-14 Last updated: 2017-11-29Bibliographically approved

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