Stimulated X-Ray Raman Scattering with Free-Electron Laser Sources
2016 (English)In: X-Ray Lasers 2014, Springer, 2016, 201-207 p.Chapter in book (Refereed)
Stimulated electronic x-ray Raman scattering is the building block for several proposed x-ray pump probe techniques, that would allow the study of electron dynamics at unprecedented timescales.We present high spectral resolution data on stimulated electronic x-ray Raman scattering in a gas sample of neon using a self-amplified spontaneous emission x-ray free-electron laser. Despite the limited spectral coherence and broad bandwidth of these sources, high-resolution spectra can be obtained by statistical methods, opening the path to coherent stimulated x-ray Raman spectroscopy. An extension of these ideas to molecules and the results of a recent experiment in CO are discussed.
Place, publisher, year, edition, pages
Springer, 2016. 201-207 p.
, Springer Proceedings in Physics, ISSN 0930-8989 ; 169
Electrons, Free electron lasers, Neon, Pumping (laser), Raman scattering, Raman spectroscopy, Spectral resolution, Electron dynamics, High spectral resolution, High-resolution spectra, Pump-probe technique, Self-amplified spontaneous emission, Spectral coherence, X-ray free electron lasers, X-ray raman scatterings
Atom and Molecular Physics and Optics
IdentifiersURN: urn:nbn:se:kth:diva-194079DOI: 10.1007/978-3-319-19521-6_26ISI: 000378036600026ScopusID: 2-s2.0-84951860407ISBN: 978-3-319-19521-6ISBN: 978-3-319-19520-9OAI: oai:DiVA.org:kth-194079DiVA: diva2:1037235
QC 201610172016-10-142016-10-142016-10-17Bibliographically approved