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Crystallography as Forensic Tool for Understanding Electrolyte Degradation in Dye-sensitized Solar Cells
KTH, School of Chemical Science and Engineering (CHE), Chemistry, Applied Physical Chemistry.ORCID iD: 0000-0001-5115-4593
KTH, School of Electrical Engineering (EES), Micro and Nanosystems.ORCID iD: 0000-0003-3452-6361
KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
KTH, School of Chemical Science and Engineering (CHE), Chemistry, Applied Physical Chemistry.
2017 (English)In: CHEMISTRYSELECT, ISSN 2365-6549, Vol. 2, no 4, p. 1675-1680Article in journal (Refereed) Published
Abstract [en]

The precipitation of solid compounds from model electrolytes for liquid dye-sensitized solar cells has a story to tell regarding decomposition processes to be expected in such systems. Of course, the crystal lattice energy for a specific crystalline compounds plays a role in what compound that will eventually precipitate, but the compounds nevertheless serve as indicators for what type of processes that take place in the solar cell electrolytes upon ageing. From the compounds isolated in this study we learn that both ligand exchange processes, double-salt precipitation and oxidation are degradation processes that should not be overlooked when formulating efficient and stable electrolytes for this type of electrochemical system.

Place, publisher, year, edition, pages
WILEY-V C H VERLAG GMBH , 2017. Vol. 2, no 4, p. 1675-1680
Keywords [en]
Crystallography, Dye-sensitized solar cells, Forensics
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:kth:diva-205131DOI: 10.1002/slct.201601756ISI: 000395533900043OAI: oai:DiVA.org:kth-205131DiVA, id: diva2:1096400
Note

QC 20170517

Available from: 2017-05-17 Created: 2017-05-17 Last updated: 2017-05-17Bibliographically approved

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Gao, JiajiaFischer, Andreas C.Svensson, Per H.Kloo, Lars

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