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Electrocatalytic water oxidation by copper(II) complexes containing a tetra- or pentadentate amine-pyridine ligand
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2017 (English)In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 53, no 31, p. 4374-4377Article in journal (Refereed) Published
Abstract [en]

Two water soluble copper(ii) complexes containing amine-pyridine ligands were found to be catalytically active for water oxidation reactions in basic solutions, with observed rate constants of 13.1-18.7 s−1. These complexes are robust in basic solutions and displayed good stability over 5 h of electrolysis in pH 11.5 phosphate buffer at 1.4 V vs. NHE.

Place, publisher, year, edition, pages
Royal Society of Chemistry , 2017. Vol. 53, no 31, p. 4374-4377
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Chemical Sciences
Identifiers
URN: urn:nbn:se:kth:diva-207428DOI: 10.1039/C7CC00332CISI: 000399729100020Scopus ID: 2-s2.0-85017558038OAI: oai:DiVA.org:kth-207428DiVA, id: diva2:1098278
Note

Funding details: 21373040, NSFC, National Natural Science Foundation of China; Funding details: 21673028, NSFC, National Natural Science Foundation of China; Funding details: VR, Vetenskapsrådet; Funding text: We are grateful to the Basic Research Program of China (No. 2014CB239402), the National Natural Science Foundation of China (No. 21373040 and 21673028), the Swedish Energy Agency, the Swedish Research Council and the K and A Wallenberg Foundation for financial support of this work.

QC 20170523

Available from: 2017-05-23 Created: 2017-05-23 Last updated: 2017-05-23Bibliographically approved

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