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Far-Zone Resonant Energy Transfer in X-ray Photoemission as a Structure Determination Tool
KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology. Siberian Federal University, Russian Federation.
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2017 (English)In: Journal of Physical Chemistry Letters, ISSN 1948-7185, E-ISSN 1948-7185, Vol. 8, no 12, 2730-2734 p.Article in journal (Refereed) Published
Abstract [en]

Near-zone Förster resonant energy transfer is the main effect responsible for excitation energy flow in the optical region and is frequently used to obtain structural information. In the hard X-ray region, the Förster law is inadequate because the wavelength is generally shorter than the distance between donors and acceptors; hence, far-zone resonant energy transfer (FZRET) becomes dominant. We demonstrate the characteristics of X-ray FZRET and its fundamental differences with the ordinary near-zone resonant energy-transfer process in the optical region by recording and analyzing two qualitatively different systems: high-density CuO polycrystalline powder and SF6 diluted gas. We suggest a method to estimate geometrical structure using X-ray FZRET employing as a ruler the distance-dependent shift of the acceptor core ionization potential induced by the Coulomb field of the core-ionized donor.

Place, publisher, year, edition, pages
American Chemical Society (ACS), 2017. Vol. 8, no 12, 2730-2734 p.
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URN: urn:nbn:se:kth:diva-210274DOI: 10.1021/acs.jpclett.7b00835ISI: 000403741800030Scopus ID: 2-s2.0-85020839714OAI: oai:DiVA.org:kth-210274DiVA: diva2:1118222
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QC 20170630

Available from: 2017-06-30 Created: 2017-06-30 Last updated: 2017-07-11Bibliographically approved

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