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Temperature dependence of electrocatalytic water oxidation: a triple device model with a photothermal collector and photovoltaic cell coupled to an electrolyzer
KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
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2017 (English)In: Faraday discussions (Online), ISSN 1359-6640, E-ISSN 1364-5498, Vol. 198, 169-179 p.Article in journal (Refereed) Published
Abstract [en]

A water oxidation electrocatalyst with high activity is essential for promoting the overall efficiency of an integrated water splitting device. Herein, by investigating the prominent temperature dependence of electrocatalytic water oxidation catalyzed by first row transition metal oxides, we present how to elevate the operating temperature of the electrolyzer as an effective and universal method to improve its electrocatalytic performance. Consequently, a triple device model combining a photothermal collector with a photovoltaic (PV) cell coupled to a water splitting device is proposed to realize the comprehensive and efficient utilization of solar energy: solar heat + PV + electrolyzer.

Place, publisher, year, edition, pages
Royal Society of Chemistry, 2017. Vol. 198, 169-179 p.
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:kth:diva-210431DOI: 10.1039/c6fd00206dISI: 000402870300010PubMedID: 28276546OAI: oai:DiVA.org:kth-210431DiVA: diva2:1119185
Funder
Swedish Energy AgencyKnut and Alice Wallenberg FoundationSwedish Research Council
Note

QC 20170703

Available from: 2017-07-03 Created: 2017-07-03 Last updated: 2017-07-03Bibliographically approved

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