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Metal-organic frameworks (ZIF-67) as efficient cocatalysts for photocatalytic reduction of CO2: The role of the morphology effect
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2018 (English)In: Journal of Materials Chemistry A, ISSN 2050-7488, Vol. 6, no 11, p. 4768-4775Article in journal (Refereed) Published
Abstract [en]

Metal-organic frameworks (MOFs), ZIF-67, with different morphologies were synthesized via a solvent-induced method at room temperature. The photocatalytic performances towards the reduction of CO2 were evaluated by using ZIF-67 materials as cocatalysts cooperating with a ruthenium-based complex as the photosensitizer. It has been demonstrated that the two-dimensional ZIF-67 with a leaf-like morphology exhibited the best photocatalytic activity and stability due to the highest CO2 adsorption capability and efficient electron transfer from the excited [Ru(bpy)3]2+ to ZIF-67.

Place, publisher, year, edition, pages
Royal Society of Chemistry, 2018. Vol. 6, no 11, p. 4768-4775
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:kth:diva-225022DOI: 10.1039/c8ta00154eScopus ID: 2-s2.0-85043785595OAI: oai:DiVA.org:kth-225022DiVA, id: diva2:1193894
Funder
Swedish Energy AgencyKnut and Alice Wallenberg Foundation
Note

QC 20180328

Available from: 2018-03-28 Created: 2018-03-28 Last updated: 2018-03-28Bibliographically approved

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