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Multidimensional resonant nonlinear spectroscopy with coherent broadband x-ray pulses
Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.;Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA..
Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA..
Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA..ORCID iD: 0000-0002-2288-2548
KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology. Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.;KTH Royal Inst Technol, Sch Biotechnol, Dept Theoret Chem & Biol, S-10691 Stockholm, Sweden..ORCID iD: 0000-0002-6706-651X
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2016 (English)In: Physica Scripta, ISSN 0031-8949, E-ISSN 1402-4896, Vol. T169, article id 014002Article in journal (Refereed) Published
Abstract [en]

New x-ray free electron laser (XFEL) and high harmonic generation (HHG) light sources are capable of generating short and intense pulses that make x-ray nonlinear spectroscopy possible. Multidimensional spectroscopic techniques, which have long been used in the nuclear magnetic resonance, infrared, and optical regimes to probe the electronic structure and nuclear dynamics of molecules by sequences of short pulses with variable delays, can thus be extended to the attosecond x-ray regime. This opens up the possibility of probing core-electronic structure and couplings, the real-time tracking of impulsively created valence-electronic wavepackets and electronic coherences, and monitoring ultrafast processes such as nonadiabatic electron-nuclear dynamics near conical-intersection crossings. We survey various possible types of multidimensional x-ray spectroscopy techniques and demonstrate the novel information they can provide about molecules.

Place, publisher, year, edition, pages
IOP PUBLISHING LTD , 2016. Vol. T169, article id 014002
Keywords [en]
x-ray, spectroscopy, Raman, four-wave-mixing
National Category
Physical Sciences
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URN: urn:nbn:se:kth:diva-242662DOI: 10.1088/0031-8949/T169/1/014002ISI: 000413519600002Scopus ID: 2-s2.0-85021180184OAI: oai:DiVA.org:kth-242662DiVA, id: diva2:1291360
Note

QC 20190225

Available from: 2019-02-25 Created: 2019-02-25 Last updated: 2019-02-25Bibliographically approved

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Hua, Weijie

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