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Contrasting controls on hydrogeochemistry of arsenic-enriched groundwater in the homologous tectonic settings of Andean and Himalayan basin aquifers, Latin America and South Asia
IIT, Dept Geol & Geophys, Kharagpur 721302, W Bengal, India..
IIT, Dept Geol & Geophys, Kharagpur 721302, W Bengal, India..ORCID iD: 0000-0002-0555-0875
KTH, School of Architecture and the Built Environment (ABE), Sustainable development, Environmental science and Engineering.ORCID iD: 0000-0003-4350-9950
USQ, Sch Civil Engn & Surveying, Toowoomba, Qld 4350, Australia.;USQ, Int Ctr Appl Climate Sci, Toowoomba, Qld 4350, Australia..
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2019 (English)In: SCIENCE OF THE TOTAL ENVIRONMENT, Vol. 689, p. 1370-1387Article in journal (Refereed) Published
Abstract [en]

High groundwater arsenic (As) across the globe has been one of the most well researched environmental concerns during the last two decades. Consequently, a large scientific knowledge-base has been developed on As distributions from local to global scales. However, differences in bulk sediment As concentrations cannot account for the As concentration variability in groundwater. Instead, in general, only aquifers in sedimentary basins adjacent to mountain chains (orogenic foreland basins) along continental convergent tectonic margins are found to be As enriched. We illustrate this association by integrating observations from long-term studies of two of the largest orogenic systems (i.e., As sources) and the aquifers in their associated foreland basins (As sinks), which are located in opposite hemispheres and experience distinct differences in climate and land-use patterns. The Andean orogenic system of South America (AB), an active continental margin, is in principle a modern analogue of the Himalayan orogenic system associated with the Indus-Ganges-Brahmaputra river systems in South Asia (HB). In general, the differences in hydrogeochemistry between AB and HB groundwaters are conspicuous. Major-solute composition of the arid, oxic AB groundwater exhibits a mixed-ion hydrochemical facies dominated by Na-Ca-Cl-SO4-HCO3. Molar calculations and thermodynamic modeling show that although groundwater of AB is influenced by cation exchange, its hydrochemical evolution is predominated by feldspar dissolution and relationships with secondary clays. In contrast, humid, strongly reducing groundwater of HB is dominated by Ca-HCO3 facies, suggestive of calcite dissolution, along with some weathering of silicates (monosiallitization). This work demonstrates that although hydrogeochemical evolutionary trends may vary with local climate and lithology, the fundamental similarities in global tectonic settings can still lead to the elevated concentrations of groundwater As.

Place, publisher, year, edition, pages
ELSEVIER , 2019. Vol. 689, p. 1370-1387
Keywords [en]
Tectonism, Groundwater, Arsenic, Hydrogeochemistry, Land-use pattern
National Category
Environmental Management
Identifiers
URN: urn:nbn:se:kth:diva-260156DOI: 10.1016/j.scitotenv.2019.05.444ISI: 000482379400131PubMedID: 31466173Scopus ID: 2-s2.0-85069644746OAI: oai:DiVA.org:kth-260156DiVA, id: diva2:1356215
Note

QC 20191001

Available from: 2019-10-01 Created: 2019-10-01 Last updated: 2019-10-01Bibliographically approved

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Bhattacharya, ProsunRamos Ramos, Oswaldo EduardoOrmachea Muñoz, MauricioQuino Lima, IsraelThunvik, Roger

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Mukherjee, AbhijitBhattacharya, ProsunRamos Ramos, Oswaldo EduardoOrmachea Muñoz, MauricioQuino Lima, IsraelThunvik, Roger
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