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Accelerated Chemoselective Reactions to Sequence-Controlled Heterolayered Dendrimers
KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Fibre- and Polymer Technology, Coating Technology.ORCID iD: 0000-0001-6112-0450
KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Fibre- and Polymer Technology, Coating Technology.ORCID iD: 0000-0002-8474-9478
KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Fibre- and Polymer Technology, Coating Technology.ORCID iD: 0000-0002-9200-8004
2020 (English)In: Journal of the American Chemical Society, ISSN 0002-7863, E-ISSN 1520-5126Article in journal (Refereed) Published
Abstract [en]

Chemoselective reactions are a highly desirable approach to generate well-defined functional macromolecules. Their extraordinary efficiency and selectivity enable the development of flawless structures, such as dendrimers, with unprecedented structure-to-property capacity but with typically tedious synthetic protocols. Here we demonstrate the potency of chemoselective reactions to accomplish sequence-controlled heterolayered dendrimers. An accurate accelerated design of bis-MPA monomers with orthogonally complementary moieties and a wisely selected chemical toolbox generated highly complex monodisperse dendrimers through simplified protocols. The versatility of the strategy was proved by obtaining different dendritic families with different properties after altering the order of addition of the monomers. Moreover, we evaluated the feasibility of the one-pot approach toward these heterolayered dendrimers as proof-of-concept.

Place, publisher, year, edition, pages
American Chemical Society , 2020.
National Category
Polymer Chemistry
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URN: urn:nbn:se:kth:diva-267981DOI: 10.1021/jacs.9b11726ISI: 000509425600048PubMedID: 31895981Scopus ID: 2-s2.0-85078546164OAI: oai:DiVA.org:kth-267981DiVA, id: diva2:1420912
Note

QC 20200401

Available from: 2020-04-01 Created: 2020-04-01 Last updated: 2020-04-01Bibliographically approved

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Garcia Gallego, SandraAndrén, Oliver C. J.Malkoch, Michael

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