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Geometrical aspects of alpha dose rates from UO2 based fuels
Chalmers Univ Technol, Nucl Chem Ind Mat Recycling, SE-41296 Gothenburg, Sweden..
KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Chemistry, Applied Physical Chemistry.ORCID iD: 0000-0003-0663-0751
Chalmers Univ Technol, Nucl Chem Ind Mat Recycling, SE-41296 Gothenburg, Sweden..
Chalmers Univ Technol, Nucl Chem Ind Mat Recycling, SE-41296 Gothenburg, Sweden.;Swedish Nucl Fuel & Waste Management Co, SE-10124 Stockholm, Sweden..
2022 (English)In: Radiation Physics and Chemistry, ISSN 0969-806X, E-ISSN 1879-0895, Vol. 199, p. 110336-, article id 110336Article in journal (Refereed) Published
Abstract [en]

Models for calculating dose rates of spherical particles as well as in fuel cracks are important for radionuclide source term estimations. Dose rates from UO2 based fuels were calculated for planar, spherical, and crack geometries. The escape probability for a-particles in spherical UO2 particles was derived as a continuous equation. The dose rate increased with increasing spherical radius due to the decreasing relative volume of the surrounding water layer. The model produced escape probabilities that were closely predicted by the theoretical derivation. It was shown that the dose rate in water filled fuel cracks with width smaller than the range of an alpha-particle led to dissolution rates that were lower per unit surface area.

Place, publisher, year, edition, pages
Elsevier BV , 2022. Vol. 199, p. 110336-, article id 110336
Keywords [en]
UO2, Alpha particles, Radiolytic oxidation, Dose rate, Fuel cracks, Spherical geometry
National Category
Subatomic Physics Energy Systems
Identifiers
URN: urn:nbn:se:kth:diva-316443DOI: 10.1016/j.radphyschem.2022.110336ISI: 000833539800009Scopus ID: 2-s2.0-85132502913OAI: oai:DiVA.org:kth-316443DiVA, id: diva2:1688273
Note

QC 20220818

Available from: 2022-08-18 Created: 2022-08-18 Last updated: 2022-08-18Bibliographically approved

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Jonsson, Mats

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CiteExportLink to record
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  • apa
  • ieee
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  • Other style
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  • de-DE
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Output format
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  • rtf