kth.sePublications
Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Optically controlling the competition between spin flips and intersite spin transfer in a Heusler half-metal on sub-100-fs time scales
JILA, University of Colorado Boulder, 440 UCB, Boulder, CO 80309, USA..
JILA, University of Colorado Boulder, 440 UCB, Boulder, CO 80309, USA..
Division of Materials Theory, Department of Physics and Astronomy, Uppsala University, Box-516, SE 75120, Sweden..
JILA, University of Colorado Boulder, 440 UCB, Boulder, CO 80309, USA..
Show others and affiliations
2023 (English)In: Science Advances, E-ISSN 2375-2548, Vol. 9, no 45, p. 1428-Article in journal (Refereed) Published
Abstract [en]

The direct manipulation of spins via light may provide a path toward ultrafast energy-efficient devices. However, distinguishing the microscopic processes that can occur during ultrafast laser excitation in magnetic alloys is challenging. Here, we study the Heusler compound Co2MnGa, a material that exhibits very strong light-induced spin transfers across the entire M-edge. By combining the element specificity of extreme ultraviolet high-harmonic probes with time-dependent density functional theory, we disentangle the competition between three ultrafast light-induced processes that occur in Co2MnGa: same-site Co-Co spin transfer, intersite Co-Mn spin transfer, and ultrafast spin flips mediated by spin-orbit coupling. By measuring the dynamic magnetic asymmetry across the entire M-edges of the two magnetic sublattices involved, we uncover the relative dominance of these processes at different probe energy regions and times during the laser pulse. Our combined approach enables a comprehensive microscopic interpretation of laser-induced magnetization dynamics on time scales shorter than 100 femtoseconds.

Place, publisher, year, edition, pages
American Association for the Advancement of Science (AAAS) , 2023. Vol. 9, no 45, p. 1428-
National Category
Condensed Matter Physics Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:kth:diva-340110DOI: 10.1126/sciadv.adi1428ISI: 001142520500002PubMedID: 37948525Scopus ID: 2-s2.0-85176433605OAI: oai:DiVA.org:kth-340110DiVA, id: diva2:1815197
Note

QC 20231128

Available from: 2023-11-28 Created: 2023-11-28 Last updated: 2024-02-21Bibliographically approved

Open Access in DiVA

No full text in DiVA

Other links

Publisher's full textPubMedScopus

Authority records

Delin, Anna

Search in DiVA

By author/editor
Delin, Anna
By organisation
SeRC - Swedish e-Science Research CentreMaterials and Nanophysics
In the same journal
Science Advances
Condensed Matter PhysicsAtom and Molecular Physics and Optics

Search outside of DiVA

GoogleGoogle Scholar

doi
pubmed
urn-nbn

Altmetric score

doi
pubmed
urn-nbn
Total: 19 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf