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Kapitza Stabilization of Quantum Critical Order
Nordita SU.
Department of Materials, ETH Zürich, Zürich, CH-8093, Switzerland.
Department of Materials, ETH Zürich, Zürich, CH-8093, Switzerland.
Laboratory for Quantum Magnetism, Institute of Physics, École Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland.
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2024 (English)In: Physical Review X, E-ISSN 2160-3308, Vol. 14, no 2, article id 021016Article in journal (Refereed) Published
Abstract [en]

Dynamical perturbations modify the states of classical systems in surprising ways and give rise to important applications in science and technology. For example, Floquet engineering exploits the possibility of band formation in the frequency domain when a strong, periodic variation is imposed on parameters such as spring constants. We describe here Kapitza engineering, where a drive field oscillating at a frequency much higher than the characteristic frequencies for the linear response of a system changes the potential energy surface so much that maxima found at equilibrium become local minima, in precise analogy to the celebrated Kapitza pendulum where the unstable inverted configuration, with the mass above rather than below the fulcrum, actually becomes stable. Our starting point is a quantum field theory of the Ginzburg-Devonshire type, suitable for many condensed matter systems, including particularly ferroelectrics and quantum paralectrics. We show that an off-resonance oscillatory electric field generated by a laser-driven terahertz source can induce ferroelectric order in the quantum-critical limit. Heating effects are estimated to be manageable using pulsed radiation; "hidden"radiation-induced order can persist to low temperatures without further pumping due to stabilization by strain. We estimate the Ginzburg-Devonshire free-energy coefficients in SrTiO3 using density-functional theory and the stochastic self-consistent harmonic approximation accelerated by a machine-learned force field. Although we find that SrTiO3 is not an optimal choice for Kapitza stabilization, we show that scanning for further candidate materials can be performed at the computationally convenient density-functional theory level. We suggest second harmonic generation, soft-mode spectroscopy, and x-ray diffraction experiments to characterize the induced order.

Place, publisher, year, edition, pages
American Physical Society (APS) , 2024. Vol. 14, no 2, article id 021016
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:kth:diva-346392DOI: 10.1103/PhysRevX.14.021016ISI: 001405618800001Scopus ID: 2-s2.0-85191400975OAI: oai:DiVA.org:kth-346392DiVA, id: diva2:1857586
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QC 20250212

Available from: 2024-05-14 Created: 2024-05-14 Last updated: 2025-02-12Bibliographically approved

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Balatsky, Alexander V.

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