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Parameter dependencies in multicycle THz generation with tunable high-energy pulse trains in large-aperture crystals
Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci CFEL, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, Luruper Chaussee 149, D-22761 Hamburg, Germany.;Max Planck Sch Photon, Hans Knoll Str 1, D-07745 Jena, Germany..
Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci CFEL, D-22607 Hamburg, Germany..
Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci CFEL, D-22607 Hamburg, Germany.;Paul Scherrer Inst, Forsch Str 111, CH-5232 Villigen, Switzerland..
Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci CFEL, D-22607 Hamburg, Germany.;Shanghai Jiao Tong Univ, Tsung Dao Lee Inst, Shanghai 200240, Peoples R China..
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2024 (English)In: Nonlinear Frequency Generation And Conversion:Materials And Devices Xxiii / [ed] Schunemann, P G, SPIE-Intl Soc Optical Eng , 2024, Vol. 12869, article id 128690MConference paper, Published paper (Refereed)
Abstract [en]

Efficiencies of nonlinear optical-to-terahertz (THz) conversion below one percent remain a limiting factor for applications of multicycle THz radiation like THz-driven acceleration and inspired the use of multi-line pump spectra. To overcome the difficulty of phase stabilization of multiple narrowband sources required by the multi-line approach, we exploit its temporal analog, i.e., regular pulse trains with THz repetition rate, in which the THz waves generated by rectifying the individual pulses add coherently. The optical setup producing the pulse trains consists of motorized interferometers and enables precise control over the pulse train parameters like pulse spacing and amplitude. It is operated with a laser providing 400 fs pulses and energies of up to 110 mJ, which is the highest yet attempted for a pulse-train-type experiment. Opposed to earlier work, pulse division is done after amplification making the system more flexible in terms of tuning the pulse number. We present initial results of an experimental campaign of multicycle THz generation in custom periodically-poled crystals with large-apertures up to 10x20 mm(2). The available pump energy allows filling these apertures at high fluences, promising increased THz yields. We investigate the dependence of the conversion efficiency on the single pulse duration and aim to find the optimum pulse number for different crystal lengths to determine the efficiency limitations in a regime avoiding laser-induced damage. Since crystal length and pulse number define the bandwidth of the THz pulses, this work demonstrates a path to an optimized THz source tunable to different requirements of applications.

Place, publisher, year, edition, pages
SPIE-Intl Soc Optical Eng , 2024. Vol. 12869, article id 128690M
Series
Proceedings of SPIE, ISSN 0277-786X
Keywords [en]
Multicycle, terahertz, THz generation, nonlinear conversion, pulse trains
National Category
Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:kth:diva-347910DOI: 10.1117/12.3003195ISI: 001211851200019Scopus ID: 2-s2.0-85190547444OAI: oai:DiVA.org:kth-347910DiVA, id: diva2:1871545
Conference
Conference on Nonlinear Frequency Generation and Conversion - Materials and Devices XXIII, JAN 29-31, 2024, San Francisco, CA
Note

QC 20240617

Part of ISBN 978-1-5106-6999-4, 978-1-5106-6998-7

Available from: 2024-06-17 Created: 2024-06-17 Last updated: 2025-03-28Bibliographically approved

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Zukauskas, AndriusCanalias, CarlotaPasiskevicius, ValdasLaurell, Fredrik

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