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Resonant inelastic soft X-ray scattering studies of U(VI) reduction on iron surfaces
Uppsala Universitet. (Fysik och Astronomi)
Uppsala Universitet.
Uppsala Universitet.
Uppsala Universitet. (Materialfysik)
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2004 (English)In: Materials Research Society Symposium Proceedings, ISSN 0272-9172, E-ISSN 1946-4274, Vol. 807, no Scientific Basis for Nuclear Waste Management XXVII, 113-118 p.Article in journal (Refereed) Published
Abstract [en]

The authors report on the spectroscopic anal. of several samples relevant to the processes governing the behavior of oxidized U species in groundwater solns. under anoxic conditions. Both Fe samples with different times of exposure to the U(IV) soln. and Fe metal-soln. interfaces in the liq. cell ex-situ and in-situ, resp. Resonant inelastic soft x-ray scattering is sensitive to the chem. state of U. The measurements were performed at a no. of energies of the primary photon beam across the U 5d absorption edge. The results unambiguously indicate the redn. of U(VI) to U(IV) on the Fe surface. [on SciFinder(R)]

Place, publisher, year, edition, pages
2004. Vol. 807, no Scientific Basis for Nuclear Waste Management XXVII, 113-118 p.
Keyword [en]
X ray scattering U redn iron spent fuel repository
National Category
Natural Sciences
Identifiers
URN: urn:nbn:se:kth:diva-78472ISI: 000225038400019OAI: oai:DiVA.org:kth-78472DiVA: diva2:492550
Note
CAPLUS AN 2004:922502(Journal). QC 20120306Available from: 2012-02-08 Created: 2012-02-08 Last updated: 2017-12-08Bibliographically approved

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