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Photocatalytic H-2 production in aqueous solution with host-guest inclusions formed by insertion of an FeFe-hydrogenase mimic and an organic dye into cyclodextrins
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2012 (English)In: Energy & Environmental Science, ISSN 1754-5692, E-ISSN 1754-5706, Vol. 5, no 8, 8220-8224 p.Article in journal (Refereed) Published
Abstract [en]

Bio-inspired noble-metal-free supramolecular systems were constructed by host-guest inclusions of an FeFe-hydrogenase mimic and an organic dye into cyclodextrins respectively, which give typically a ninefold increase in the TON, a sixteenfold enhancement in the quantum efficiency, and a threefold extension in lifetime as compared to the same system in the absence of cyclodextrin for photocatalytic H-2 production in aqueous solution.

Place, publisher, year, edition, pages
2012. Vol. 5, no 8, 8220-8224 p.
Keyword [en]
Beta-Cyclodextrin, Active-Site, Alpha-Cyclodextrin, Iron Hydrogenase, Model Complexes, Rose-Bengal, Water, Derivatives, Catalyst, Systems
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:kth:diva-101753DOI: 10.1039/c2ee22109hISI: 000306571800015Scopus ID: 2-s2.0-84864214302OAI: oai:DiVA.org:kth-101753DiVA: diva2:549051
Funder
Swedish Research CouncilKnut and Alice Wallenberg Foundation
Note

QC 20120903

Available from: 2012-09-03 Created: 2012-09-03 Last updated: 2017-12-07Bibliographically approved

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Sun, Licheng

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