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Simple nickel-based catalyst systems combined with graphitic carbon nitride for stable photocatalytic hydrogen production in water
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2012 (English)In: ChemSusChem, ISSN 1864-5631, Vol. 5, no 11, 2133-2138 p.Article in journal (Refereed) Published
Abstract [en]

A molecular catalyst system containing only earth-abundant elements is combined with g-C3N4 as photosensitizer. The in situ generated complexes serve as catalysts for visible-light-driven H2 production in aqueous solution, and do not require organic solvent or a Brønsted acid. H2 evolution from the Ni-based catalyst system can be maintained for over 60 h, demonstrating that the combination is a promising approach to improve the lifetimes of molecular catalysts towards photochemical H2 production.

Place, publisher, year, edition, pages
2012. Vol. 5, no 11, 2133-2138 p.
Keyword [en]
carbon nitrides, hydrogen production, nickel, photocatalysis, water splitting
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:kth:diva-108036DOI: 10.1002/cssc.201200490ISI: 000311056800004Scopus ID: 2-s2.0-84869455731OAI: oai:DiVA.org:kth-108036DiVA: diva2:579432
Funder
Knut and Alice Wallenberg Foundation
Note

QC 20121220

Available from: 2012-12-20 Created: 2012-12-19 Last updated: 2012-12-20Bibliographically approved

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Sun, Licheng

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