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Atmospheric water droplets can catalyse atom pair break-up via surface-induced resonance repulsion
KTH, School of Industrial Engineering and Management (ITM), Materials Science and Engineering, Flerskalig materialmodellering.
KTH, School of Industrial Engineering and Management (ITM), Materials Science and Engineering, Flerskalig materialmodellering.ORCID iD: 0000-0002-9050-5445
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2013 (English)In: Europhysics letters, ISSN 0295-5075, E-ISSN 1286-4854, Vol. 101, no 4, 43002- p.Article in journal (Refereed) Published
Abstract [en]

We present the theory for a retarded resonance interaction between two identical atoms near a dielectric surface. In free space the resonance interaction between isotropically excited atom pairs is attractive at all atom-atom separations. We illustrate numerically how this interaction between oxygen, sulphur, hydrogen, or nitrogen atom pairs may turn repulsive near water droplets. The results provide evidence of a mechanism causing excited state atom pair breakage to occur in the atmosphere near water droplets.

Place, publisher, year, edition, pages
2013. Vol. 101, no 4, 43002- p.
Keyword [en]
Correlated Molecular Calculations, Dipole-Dipole Interaction, Gaussian-Basis Sets, Microcavity, Energy
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Identifiers
URN: urn:nbn:se:kth:diva-120314DOI: 10.1209/0295-5075/101/43002ISI: 000315999100007Scopus ID: 2-s2.0-84874905845OAI: oai:DiVA.org:kth-120314DiVA: diva2:614298
Funder
Swedish Research Council, C0485101 70529001
Note

QC 20130404

Available from: 2013-04-04 Created: 2013-04-04 Last updated: 2017-12-06Bibliographically approved

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Persson, Clas

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