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Photoemission and density functional theory study of Ge(100): Clean surface and Yb-induced (2x4) reconstruction
KTH, School of Industrial Engineering and Management (ITM), Materials Science and Engineering, Applied Material Physics.
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2013 (English)In: Surface Science, ISSN 0039-6028, E-ISSN 1879-2758, Vol. 615, 88-96 p.Article in journal (Refereed) Published
Abstract [en]

Clean and metal-adsorbed (100) surfaces of group-IV semiconductors, such as Si and Ge, often exhibit electronically and structurally similar reconstructions. However, the fundamental bulk properties of group-IV materials can have an impact on particular features of such systems, which are related, e.g., to final-state relaxation in photoemission and thus determine their spectral line shape. Here we have studied Yb/Ge(100)(2 x 4) reconstruction as well as clean Ge(100) surface by high-resolution photoelectron spectroscopy and ab initio calculations. An atomic geometry of both surfaces is thoroughly investigated. A detailed analysis of Ge 3d core-level photoemission, atomic origins of surface-shifted components, and final-state screening effects is presented. In particular, it is demonstrated that the core-hole screening plays an essential role in Ge 3d measurements, and that its amount in the complete screening model correlates well with the core-level binding energy of respective Ge atoms in the initial state. The results are discussed in the proper context of related reconstructions on Si(100).

Place, publisher, year, edition, pages
Elsevier, 2013. Vol. 615, 88-96 p.
Keyword [en]
Germanium, Ytterbium, Photoelectron spectroscopy, DFT calculation, Atomic structure, Surface core-level shift
National Category
Physical Sciences Chemical Sciences
Identifiers
URN: urn:nbn:se:kth:diva-125542DOI: 10.1016/j.susc.2013.04.010ISI: 000321409400012Scopus ID: 2-s2.0-84878801903OAI: oai:DiVA.org:kth-125542DiVA: diva2:640261
Funder
EU, FP7, Seventh Framework Programme, 312284
Note

QC 20130813

Available from: 2013-08-13 Created: 2013-08-09 Last updated: 2017-12-06Bibliographically approved

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CiteExportLink to record
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Citation style
  • apa
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  • vancouver
  • Other style
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Language
  • de-DE
  • en-GB
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  • nn-NB
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  • Other locale
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Output format
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