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Coordination Nature of Phase Separation in Oxide Melts
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2013 (English)In: Glass Physics and Chemistry, ISSN 1087-6596, E-ISSN 1608-313X, Vol. 39, no 4, 431-443 p.Article in journal (Refereed) Published
Abstract [en]

The behavior of uranium oxide-silica, zirconia-alumina, zirconia-iron oxide, uranium oxideiron oxide, zirconia-alumina-iron oxide, and uranium oxide-iron oxide-zirconia melts was experimentally investigated in the air. The existence of two-phase fluids in these systems was confirmed. It is proposed that the reason for the phase separation is the formation of complexes with the general formula x[M3+O8/2] [Me4+O8/2]. The influence of a complex concentration on the density and surface tension of melts in the ZrO2-Al2O3 system was demonstrated.

Place, publisher, year, edition, pages
2013. Vol. 39, no 4, 431-443 p.
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:kth:diva-138835DOI: 10.1134/S1087659613040202ISI: 000322919700014Scopus ID: 2-s2.0-84882286248OAI: oai:DiVA.org:kth-138835DiVA: diva2:681800
Funder
EU, European Research Council
Note

QC 20140314

Available from: 2013-12-20 Created: 2013-12-20 Last updated: 2017-12-06Bibliographically approved

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Grishchenko, Dmitry
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