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Homogeneous Oxidation of Water by Iron Complexes with Macrocyclic Ligands
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2014 (English)In: Chemistry - An Asian Journal, ISSN 1861-4728, E-ISSN 1861-471X, Vol. 9, no 6, 1515-1518 p.Article in journal (Refereed) Published
Abstract [en]

The activity of eleven separated iron complexes and nine in situ-generated iron complexes towards catalytic water oxidation have been examined in aqueous solutions with Ce(NH4)(2)(NO3)(6) as the oxidant. Two iron complexes bearing tridentate and tetradentate macrocyclic ligands were found to be novel water oxidation catalysts. The one with tetradentate ligand exhibited a promising activity with a turnover number of 65 for oxygen evolution.

Place, publisher, year, edition, pages
2014. Vol. 9, no 6, 1515-1518 p.
Keyword [en]
homogeneous catalysis, iron complex, oxygen evolution, renewable resources, water splitting
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Other Chemistry Topics
Identifiers
URN: urn:nbn:se:kth:diva-147023DOI: 10.1002/asia.201400066ISI: 000336248900007Scopus ID: 2-s2.0-84901187858OAI: oai:DiVA.org:kth-147023DiVA: diva2:728428
Funder
Swedish Energy AgencySwedish Research CouncilKnut and Alice Wallenberg Foundation
Note

QC 20140624

Available from: 2014-06-24 Created: 2014-06-23 Last updated: 2017-12-05Bibliographically approved

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Sun, Licheng

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Organic ChemistryCentre of Molecular Devices, CMD
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