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Artificial photosynthesis: photosensitizer/catalyst supramolecular assemblies for light driven water oxidation
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2014 (English)In: Faraday discussions (Online), ISSN 1364-5498, E-ISSN 1359-6640, Vol. 176, 225-232 p.Article in journal (Refereed) Published
Abstract [en]

Three new supramolecular assemblies SA1-SA3 with different linkages between the photosensitizer and catalyst have been synthesized for light driven water oxidation. With flexible -CH2-CH2- chains as the linkage, the assembly SA3 displays the best performance for photocatalytic water oxidation compared with the other two assemblies, a turnover number of 34 has been obtained based on the molecular assembly SA3 in a homogeneous system. This type of assembly connected with flexible linkages represents suitable candidates to construct photoanodes for light driven water splitting in dye sensitized photoelectrochemical devices.

Place, publisher, year, edition, pages
2014. Vol. 176, 225-232 p.
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Chemical Sciences
URN: urn:nbn:se:kth:diva-164016DOI: 10.1039/c4fd00127cISI: 000350894400015ScopusID: 2-s2.0-84924661288OAI: diva2:805022
Swedish Energy AgencyKnut and Alice Wallenberg Foundation

QC 20150414

Available from: 2015-04-14 Created: 2015-04-13 Last updated: 2015-04-14Bibliographically approved

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Sun, Licheng
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