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Fragmentation of mercury compounds under ultraviolet light irradiation
Univ Oulu, Ctr Mol Mat Res, Oulu 90014, Finland..
KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology. Univ Oulu, Ctr Mol Mat Res, Oulu 90014, Finland.;Royal Inst Technol, Sch Biotechnol, Div Theoret Chem & Biol, S-10691 Stockholm, Sweden..
Univ Oulu, Ctr Mol Mat Res, Oulu 90014, Finland..
Univ Oulu, Ctr Mol Mat Res, Oulu 90014, Finland..
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2015 (English)In: Journal of Chemical Physics, ISSN 0021-9606, E-ISSN 1089-7690, Vol. 143, no 7, 074307Article in journal (Refereed) Published
Abstract [en]

Ultraviolet light induced photofragmentation of mercury compounds is studied experimentally with electron energy resolved photoelectron-photoion coincidence techniques and theoretically with computational quantum chemical methods. A high resolution photoelectron spectrum using synchrotron radiation is presented. Fragmentation of the molecule is studied subsequent to ionization to the atomic-mercury-like d orbitals. State dependent fragmentation behaviour is presented and specific reactions for dissociation pathways are given. The fragmentation is found to differ distinctly in similar orbitals of different mercury compounds.

Place, publisher, year, edition, pages
2015. Vol. 143, no 7, 074307
National Category
Atom and Molecular Physics and Optics
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URN: urn:nbn:se:kth:diva-173774DOI: 10.1063/1.4928651ISI: 000360440400029Scopus ID: 2-s2.0-84939857579OAI: oai:DiVA.org:kth-173774DiVA: diva2:855348
Note

QC 20150921

Available from: 2015-09-21 Created: 2015-09-18 Last updated: 2017-12-04Bibliographically approved

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