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Electron dynamics in the core-excited CS2 molecule revealed through resonant inelastic x-ray scattering spectroscopy
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2015 (English)In: XXIX INTERNATIONAL CONFERENCE ON PHOTONIC, ELECTRONIC, AND ATOMIC COLLISIONS (ICPEAC2015), PTS 1-12, Institute of Physics Publishing (IOPP), 2015, UNSP 112012Conference paper (Refereed)Text
Abstract [en]

We present an experimental and theoretical study of resonant inelastic x-ray scattering (RIXS) in the CS2 molecule near the S 1s edge. We show that localization of the S 1s core-hole occurs in CS2 during the RIXS process due to the orientational dephasing of interference between the waves scattering on the two sulfur atoms. Strong evolution of the RIXS profile with the excitation energy far below the first absorption resonance reflects the onset of electron dynamics triggered by a coherent excitation of multiple electronic states.

Place, publisher, year, edition, pages
Institute of Physics Publishing (IOPP), 2015. UNSP 112012
Series
, Journal of Physics Conference Series, ISSN 1742-6588 ; 635
National Category
Physical Sciences
Identifiers
URN: urn:nbn:se:kth:diva-180394DOI: 10.1088/1742-6596/635/11/112012ISI: 000366407000596ScopusID: 2-s2.0-84948807628OAI: oai:DiVA.org:kth-180394DiVA: diva2:894003
Conference
29th International Conference on Photonic, Electronic, and Atomic Collisions (ICPEAC), JUL 22-28, 2015, Toledo, SPAIN
Note

QC 20160114

Available from: 2016-01-14 Created: 2016-01-13 Last updated: 2016-01-20Bibliographically approved

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da Cruz, V. VazGelmukhanov, Faris
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ReferencesLink to record
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