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  • 1.
    Chen, Tianyang
    et al.
    MIT, Dept Chem, Cambridge, MA 02139 USA..
    Dou, Jin-Hu
    MIT, Dept Chem, Cambridge, MA 02139 USA..
    Yang, Luming
    MIT, Dept Chem, Cambridge, MA 02139 USA..
    Sun, Chenyue
    MIT, Dept Chem, Cambridge, MA 02139 USA..
    Oppenheim, Julius J.
    MIT, Dept Chem, Cambridge, MA 02139 USA..
    Li, Jian
    KTH, School of Engineering Sciences in Chemistry, Biotechnology and Health (CBH), Fibre- and Polymer Technology, Fibre Technology. Stockholm Univ, Berzelii Ctr EXSELENT Porous Mat, Dept Mat & Environm Chem, S-10691 Stockholm, Sweden..
    Dinca, Mircea
    MIT, Dept Chem, Cambridge, MA 02139 USA..
    Dimensionality Modulates Electrical Conductivity in Compositionally Constant One-, Two-, and Three-Dimensional Frameworks2022In: Journal of the American Chemical Society, ISSN 0002-7863, E-ISSN 1520-5126, Vol. 144, no 12, p. 5583-5593Article in journal (Refereed)
    Abstract [en]

    We reveal here the construction of Ni-based metal-organic frameworks (MOFs) and conjugated coordination polymers (CCPs) with different structural dimensionalities, including closely pi-stacked 1D chains (Ni-1D), aggregated 2D layers (Ni-2D), and a 3D framework (Ni-3D), based on 2,3,5,6-tetraamino-1,4-hydroquinone (TAHQ) and its various oxidized forms. These materials have the same metal-ligand composition but exhibit distinct electronic properties caused by different dimensionalities and supramolecular interactions between SBUs, ligands, and structural motifs. The electrical conductivity of these materials spans nearly 8 orders of magnitude, approaching 0.3 S/cm.

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