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  • 1. Gao, Yan
    et al.
    Ding, Xin
    Liu, Jianhui
    Wang, Lei
    KTH, School of Chemical Science and Engineering (CHE), Chemistry.
    Lu, Zhongkai
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Visible Light Driven Water Splitting in a Molecular Device with Unprecedentedly High Photocurrent Density2013In: Journal of the American Chemical Society, ISSN 0002-7863, E-ISSN 1520-5126, Vol. 135, no 11, p. 4219-4222Article in journal (Refereed)
    Abstract [en]

    A molecular water oxidation catalyst (2) has been synthesized and immobilized together with a molecular photosensitizer (1) on nanostructured TiO2 particles on FTO conducting glass, forming a photoactive anode (TiO2(1+2)). By using the TiO2(1+2) as working electrode in a three-electrode photoelectrochemical cell (PEC), visible light driven water splitting has been successfully demonstrated in a phosphate buffer solution (pH 6.8), with oxygen and hydrogen bubbles evolved respectively from the working electrode and counter electrode. By applying 0.2 V external bias vs NHE, a high photocurrent density of more than 1.7 rnA.cm(-2) has been achieved. This value is higher than any PEC devices with molecular components reported in literature.

  • 2.
    Li, Fusheng
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Fan, Ke
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Xu, Bo
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Gabrielsson, Erik
    Daniel, Quentin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. State Key Laboratory of Fine Chemicals, DUT-KTH Joint Education and Research Center on Molecular Devices, Dalian University of Technology (DUT), Dalian, China.
    Organic Dye-Sensitized Tandem Photoelectrochemical Cell for Light Driven Total Water Splitting2015In: Journal of the American Chemical Society, ISSN 0002-7863, E-ISSN 1520-5126, Vol. 137, no 28, p. 9153-9159Article in journal (Refereed)
    Abstract [en]

    Light driven water splitting was achieved by a tandem dye-sensitized photoelectrochemical cell with two photoactive electrodes. The photoanode is constituted by an organic dye L0 as photosensitizer and a molecular complex Ru1 as water oxidation catalyst on meso-porous TiO2, while the photocathode is constructed with an organic dye P1 as photoabsorber and a molecular complex Col as hydrogen generation catalyst on nanostructured NiO. By combining the photocathode and the photoanode, this tandem DS-PEC cell can split water by visible light under neutral pH conditions without applying any bias.

  • 3.
    Li, Fusheng
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Chemistry.
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Tong, Lianpeng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Daniel, Quentin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry.
    Göthelid, Mats
    KTH, School of Information and Communication Technology (ICT), Materials- and Nano Physics, Material Physics, MF.
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Immobilization of a molecular catalyst on carbon nanotubes for highly efficient electro-catalytic water oxidation2014In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 50, no 90, p. 13948-13951Article in journal (Refereed)
    Abstract [en]

    Electrochemically driven water oxidation has been performed using a molecular water oxidation catalyst immobilized on hybrid carbon nanotubes and nano-material electrodes. A high turnover frequency (TOF) of 7.6 s(-1) together with a high catalytic current density of 2.2 mA cm(-2) was successfully obtained at an overpotential of 480 mV after 1 h of bulk electrolysis.

  • 4.
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Functional Photo-electrochemical Devices for Solar Cellsand Solar Fuels Based on Molecular Components2012Doctoral thesis, comprehensive summary (Other academic)
    Abstract [en]

    This thesis concerns the development and the study of molecular functional photo-electrochemical cells (PEC) for solar cells and solar fuels.

    The first chapter gives a general introduction about photosynthesis, dye-sensitized solar cell and photo-electrochemical device for water splitting.

    The second chapter describes a TiO2-Co-catalyst electrode manufactured by a direct photo-deposition method. The electrode showed activity for electrochemical water oxidation in an electrochemical device.

    In the third chapter, a photo-electrochemical cell (PEC) with two-electrodes for visible light driven water splitting has been successfully demonstrated. One electrode was a photo-anode, which assembled a ruthenium water oxidation catalyst (complex 1) into a dye-sensitized porous nanostructured TiO2 electrode by employing a cation-exchange membrane (Nafion). The other electrode was platinum which was used as a passive cathode for proton reduction.

    In the fourth chapter, an earth abundant metal complex with an anchoring group (cobalt complex 2) was synthesized and investigated as water oxidation catalyst. This complex was further applied into a photo-anode in a PEC. The photo-anode was assembled by co-sensitization of complex 2 to a dye-sensitized porous nanostructured TiO2 electrode. The PEC device gave ca. 250 υA/cm2 photo-current and 7.2 % IPCE without applying any bias voltage, which is much higher than the reported results in the sample type of PEC. Meanwhile, we have shown that the catalytic effect is not from free cobalt ions, CoOx film or nanoparticles formed in situ by using complex 2 in the device.

    The last two chapters describe an optimization of the NiO films prepared in two steps rather than one step film and applied in p-type DSSCs. This optimized film could adsorb more dye (P1), leading to a significant light harvesting efficiency (LHE) and IPCE in DSSCs. We further combined this P1 sensitized photo-cathode with a hydrogen evolution catalyst (complex 3) and applied this photo-cathode into a PEC for visible light hydrogen evolution.

  • 5.
    Li, Lin
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Duan, Lele
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Wen, Fuyu
    Li, Can
    Wang, Mei
    Hagfeld, Anders
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Visible light driven hydrogen production from a photo-active cathode based on a molecular catalyst and organic dye-sensitized p-type nanostructured NiO2012In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 48, no 7, p. 988-990Article in journal (Refereed)
    Abstract [en]

    A molecular device with a photocathode for hydrogen generation has been successfully demonstrated, based on an earth abundant and inexpensive p-type semiconductor NiO, an organic dye P1 and a cobalt catalyst Co1.

  • 6.
    Li, Lin
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD. KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Duan, Lele
    KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD. KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Xu, Yunhua
    KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD. KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Gorlov, Mikhail
    KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD. KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Hagfeldt, Anders
    KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD. KTH, School of Chemical Science and Engineering (CHE), Chemistry, Physical Chemistry.
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD. KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    A photoelectrochemical device for visible light driven water splitting by a molecular ruthenium catalyst assembled on dye-sensitized nanostructured TiO22010In: Chemical Communications, ISSN 1359-7345, E-ISSN 1364-548X, Vol. 46, no 39, p. 7307-7309Article in journal (Refereed)
    Abstract [en]

    A photoelectrochemical device with a molecular Ru catalyst assembled via pH-modified Nafion on a dye-sensitized nanostructured TiO2 film as anode and a Pt foil as cathode has been successfully demonstrated to split water into O-2 and H-2 driven by visible light.

  • 7.
    Li, Lin
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Gibson, Elisabeth A.
    Qin, Peng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Boschloo, Gerrit
    Gorlov, Mikhail
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Hagfeldt, Anders
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Double-Layered NiO Photocathodes for p-Type DSSCs with Record IPCE2010In: Advanced Materials, ISSN 0935-9648, E-ISSN 1521-4095, Vol. 22, no 15, p. 1759-1762Article in journal (Refereed)
    Abstract [en]

    A way to achieve a high-efficiency dye-sensitized solar cell is to combine an n-type TiO2-based photoanode with a p-type photocathode in a tandem configuration. The development of an efficient photocathode is, at present, the key target. We have optimized the NiO, I-3(-)/I- p-DSSC system to obtain record photocurrent, giving 64% incident photon-to-current conversion efficiency (IPCE) and 5.48 mAcm(-2) J(SC).

  • 8.
    Li, Lin
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Li, Fusheng
    Duan, Lele
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Electrocatalytic water splitting: A bi-functional water-soluble molecular Co-based complex for both catalytic water oxidation and hydrogen generationManuscript (preprint) (Other academic)
  • 9.
    Li, Lin
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Lohse, Peter William
    Li, Fusheng
    Hagfeldt, Anders
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    A photoelectrochemical device for visible light driven water splitting with a molecular cobalt complex assembled on dye-sensitized porous nanocrystalline TiO2 electrodeManuscript (preprint) (Other academic)
  • 10.
    Lin, Li
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    LiCheng, Sun
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Electrochemical water oxidation by photo-deposited cobalt-based catalyst on a nano-structured TiO2 electrode2012In: Science China Chemistry, ISSN 1674-7291, Vol. 55, no 9, p. 1976-1981Article in journal (Refereed)
    Abstract [en]

    A cobalt-based catalyst was directly photo-deposited on the surface of a widely used n-type nano-structured semiconductor (TiO2). Different thicknesses of the TiO2 films as well as different time of photo-deposition of the Co-based catalyst on TiO2 films have been optimized. It was found that the electrode with 3 layers of TiO2 film (in 8 mu m thickness) and 1 hour photo-deposition of the cobalt-based catalyst by light irradiation from a 500 W Xenon lamp gave the highest current density (similar to 5 mA/cm(2)). Using this cobalt-modified TiO2 film as a working electrode in an electrochemical device, highly efficient water oxidation has been demonstrated in a pH 7.0 aqueous solution with low overpotential.

  • 11.
    Ning, Zhijun
    et al.
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Yuan, Chunze
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Tian, Haining
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Fu, Ying
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Ågren, Hans
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Type-II colloidal quantum dot sensitized solar cells with a thiourea based organic redox couple2012In: Journal of Materials Chemistry, ISSN 0959-9428, E-ISSN 1364-5501, Vol. 22, no 13, p. 6032-6037Article in journal (Refereed)
    Abstract [en]

    In this paper, one kind of organic electrolyte based on tetramethylthiourea is employed for quantum dot sensitized solar cells (QDSCs). By reducing the impedance between the electrolyte and the counter electrode, the fill factor of such organic electrolyte based QDSCs is significantly improved. It is possible to substantially increase the photovoltage and to reach an efficiency three times higher than that of a commonly used inorganic electrolyte. The light harvesting ability of the organic electrolyte based QDSCs is successfully extended by using type-II QDs, where the adsorption of ZnS gives an additional advantage in further enhancing the stability of the cells. It is observed that core/shell ZnSe/CdS type-II QDs give higher electron injection than CdS/ZnSe QDs, proving that the electron distribution in the QDs is important for the electron extraction. A full working mechanism of the organic redox couple for the QDSCs is proposed.

  • 12.
    Qin, Peng
    et al.
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Wiberg, Joanna
    Gibson, Elizabeth A.
    Linder, Mats
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Brinck, Tore
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Physical Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Hagfeldt, Anders
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Albinsson, Bo
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry. KTH, School of Chemical Science and Engineering (CHE), Centres, Centre of Molecular Devices, CMD.
    Synthesis and Mechanistic Studies of Organic Chromophores with Different Energy Levels for p-Type Dye-Sensitized Solar Cells2010In: The Journal of Physical Chemistry C, ISSN 1932-7447, E-ISSN 1932-7455, Vol. 114, no 10, p. 4738-4748Article in journal (Refereed)
    Abstract [en]

    A series of donor-pi-acceptor dyes with different electron-withdrawing groups were designed and synthesized for p-type dye-sensitized Solar cells. The modification of dye structures shows significant influence on the photophysical, electrochemical, and photovoltaic performance of the dyes. DSSCs based on these dyes show maximum 63% and minimum 6% of incident monochromatic photon-to-current conversion efficiencies. The two dyes with the highest (P1) and lowest (P3) efficiencies were Studied by femtosecond transient absorption spectroscopy, which shows a fast injection rate of more than (250 fs)(-1) for both dyes. Such fast injection corresponds to more than 90% injection efficiency. The photoinduced absorption Spectroscopy Study of sensitized NiO films in the presence of electrolyte showed poor regeneration of 113 due to all insufficient driving force. This, together with aggregation of the dye on the NiO film, explained the poor solar cell performance.

  • 13.
    Yuan, Chunze
    et al.
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Chen, Guanying
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology. University of Buffalo, United States; Harbin Institute of Technology, China .
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Damasco, Jossana A.
    Ning, Zhijun
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Xing, Hui
    Zhang, Tianmu
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Zeng, Hao
    Cartwright, Alexander N.
    Prasad, Paras N.
    Ågren, Hans
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Simultaneous Multiple Wavelength Upconversion in a Core-Shell Nanoparticle for Enhanced Near Infrared Light Harvesting in a Dye-Sensitized Solar Cell2014In: ACS Applied Materials and Interfaces, ISSN 1944-8244, E-ISSN 1944-8252, Vol. 6, no 20, p. 18018-18025Article in journal (Refereed)
    Abstract [en]

    The efficiency of most photovoltaic devices is severely limited by near-infrared (NIR) transmission losses. To alleviate this limitation, a new type of colloidal upconversion nanoparticles (UCNPs), hexagonal core-shell-structured beta-NaYbF4:Er3+(2%)/NaYF4:Nd3+(30%), is developed and explored in this work as an NIR energy relay material for dye-sensitized solar cells (DSSCs). These UCNPs are able to harvest light energy in multiple NIR regions, and subsequently convert the absorbed energy into visible light where the DSSCs strongly absorb. The NIR-insensitive DSSCs show compelling photocurrent increases through binary upconversion under NIR light illumination either at 785 or 980 nm, substantiating efficient energy relay by these UCNPs. The overall conversion efficiency of the DSSCs was improved with the introduction of UCNPs under simulated AM 1.5 solar irradiation.

  • 14.
    Yuan, Chunze
    et al.
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Chen, Guanying
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Damasco, Jossana
    Ning, Zhijun
    Xing, Hui
    Zhang, Tianmu
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Zeng, Hao
    Prasad, Paras N.
    Ågren, Hans
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Effective Dual-NIR-Wavelength Energy Relay of Colloidal Upconversion Nanocrystals for Dye-sensitized Solar CellsManuscript (preprint) (Other academic)
  • 15.
    Yuan, Chunze
    et al.
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Li, Lin
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Huang, Jing
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Ning, Zhijun
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Ågren, Hans
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Improving the Photocurrent in Quantum-Dot-Sensitized Solar Cells by Employing Alloy PbxCd1-xS Quantum Dots as Photosensitizers2016In: NANOMATERIALS, ISSN 2079-4991, Vol. 6, no 6, article id UNSP 97Article in journal (Refereed)
    Abstract [en]

    Ternary alloy PbxCd1-xS quantum dots (QDs) were explored as photosensitizers for quantum-dot-sensitized solar cells (QDSCs). Alloy PbxCd1-xS QDs (Pb0.54Cd0.46S, Pb0.31Cd0.69S, and Pb0.24Cd0.76S) were found to substantially improve the photocurrent of the solar cells compared to the single CdS or PbS QDs. Moreover, it was found that the photocurrent increases and the photovoltage decreases when the ratio of Pb in PbxCd1-xS is increased. Without surface protecting layer deposition, the highest short-circuit current density reaches 20 mA/cm(2) under simulated AM 1.5 illumination (100 mW/cm(2)). After an additional CdS coating layer was deposited onto the PbxCd1-xS electrode, the photovoltaic performance further improved, with a photocurrent of 22.6 mA/cm(2) and an efficiency of 3.2%.

  • 16.
    Yuan, Chunze
    et al.
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Ning, Zhijun
    Huang, Jing
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Ågren, Hans
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    A Strategy to Improve Photocurrent in Quantum Dot Sensitized Solar Cells by Employing Alloy PbxCd1-xS QDs as PhotosensitizersManuscript (preprint) (Other academic)
  • 17.
    Yuan, Chunze
    et al.
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Li, Lin
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Ning, Zhijun
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Sun, Licheng
    KTH, School of Chemical Science and Engineering (CHE), Chemistry, Organic Chemistry.
    Fu, Ying
    KTH, School of Biotechnology (BIO), Theoretical Chemistry and Biology.
    Study of CdS quantum dot solar cells directly deposited on p-type NiO photoelectrodesManuscript (preprint) (Other academic)
1 - 17 of 17
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