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Loiko, P., Agazzi, L., Kores, C. C., Dijkstra, M., Geskus, D. & Pollnau, M. (2025). Quantitative analysis of cooperative upconversion in Al2O3:Yb3+. Optical materials (Amsterdam), 162, Article ID 116798.
Open this publication in new window or tab >>Quantitative analysis of cooperative upconversion in Al2O3:Yb3+
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2025 (English)In: Optical materials (Amsterdam), ISSN 0925-3467, E-ISSN 1873-1252, Vol. 162, article id 116798Article in journal (Refereed) Published
Abstract [en]

Amorphous Al2O3 channel waveguides with different Yb3+ concentrations are fabricated by reactive co-sputtering onto thermally oxidized silicon substrates and subsequent reactive ion etching. Pump transmission and bleaching of pump absorption, luminescence spectra, luminescence-decay curves, and the dependence of luminescence intensity on pump power are measured for the transition at 1 μm from the 2F5/2 first excited state of Yb3+ and for the green upconversion luminescence from the second excited state of the single quantum systems formed by Yb3+-Yb3+ pairs. The typical spectroscopic features of cooperative upconversion are observed. Analysis by rate equations reveals that only a microscopic two-ion-class model comprising single ions and ion pairs can quantitatively explain the measured spectroscopic data, i.e., the local chemical environment must be taken into account in the analysis. The fraction of quenched ions determined from the pump-absorption measurements and the fractions of ions forming Yb3+-Yb3+ pairs and producing cooperative upconversion (CU) are found to be equivalent and increase linearly with Yb3+ concentration. It suggests that the observed phenomena of non-saturable absorption and CU are linked to each other and evoked by the same class of ions. Internal net gain in these channel waveguides under the influence of cooperative upconversion is experimentally investigated and successfully modeled by use of the two-ion-class model. This analysis delivers important spectroscopic insight for optimizing the performance of distributed-feedback lasers in these waveguides. Particularly, it will provide a route towards optimizing the Yb3+ concentration for simultaneously ensuring sufficient pump absorption and minimizing non-saturable absorption by CU-quenched Yb3+-Yb3+ pairs that would otherwise significantly increase the laser linewidth, which is the most important performance parameter of such lasers.

Place, publisher, year, edition, pages
Elsevier BV, 2025
Keywords
Cooperative processes, Optical waveguides, Rare-earth ions, Thin films, Upconversion
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-362039 (URN)10.1016/j.optmat.2025.116798 (DOI)001456240900001 ()2-s2.0-105000711090 (Scopus ID)
Note

QC 20250407

Available from: 2025-04-03 Created: 2025-04-03 Last updated: 2025-05-06Bibliographically approved
Kores, C. C., Geskus, D., Dijkstra, M. & Pollnau, M. (2020). Enhanced linewidth narrowing in a distributed-feedback resonator. In: : . Paper presented at Europhoton. , Article ID We-A2.3.
Open this publication in new window or tab >>Enhanced linewidth narrowing in a distributed-feedback resonator
2020 (English)Conference paper, Oral presentation only (Other academic)
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-287348 (URN)
Conference
Europhoton
Note

QC 20201208

Available from: 2020-12-08 Created: 2020-12-08 Last updated: 2022-06-25Bibliographically approved
Loiko, P., Agazzi, L., Kores, C. C., Dijkstra, M., Geskus, D. & Pollnau, M. (2020). Quantitative analysis of cooperative upconversion in Al2O3:Yb3+ waveguides on silicon. In: Europhoton: . Paper presented at Europhoton. , Article ID We-A2.7.
Open this publication in new window or tab >>Quantitative analysis of cooperative upconversion in Al2O3:Yb3+ waveguides on silicon
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2020 (English)In: Europhoton, 2020, article id We-A2.7Conference paper, Oral presentation only (Other academic)
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-287349 (URN)
Conference
Europhoton
Note

QC 20201208

Available from: 2020-12-08 Created: 2020-12-08 Last updated: 2022-06-25Bibliographically approved
Loiko, P., Agazzi, L., Kores, C. C., Dijkstra, M., Geskus, D. & Pollnau, M. (2020). Spectroscopy, cooperative upconversion and optical gain in amorphous al2O3:Yb3+ waveguides on silicon. In: Optics InfoBase Conference Papers: . Paper presented at CLEO: Science and Innovations, CLEO_SI 2020; Washington; United States; 10 May 2020 through 15 May 2020. The Optical Society
Open this publication in new window or tab >>Spectroscopy, cooperative upconversion and optical gain in amorphous al2O3:Yb3+ waveguides on silicon
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2020 (English)In: Optics InfoBase Conference Papers, The Optical Society , 2020Conference paper, Published paper (Refereed)
Abstract [en]

Ridge waveguides in amorphous Al2O3:Yb3+ are produced by reactive co-sputtering and reactive-ion etching. Their spectroscopic properties, optical gain, and cooperative upconversion are studied and explained based on a model of distinct ion classes.

Place, publisher, year, edition, pages
The Optical Society, 2020
Keywords
Alumina, Aluminum oxide, Optical gain, Optical waveguides, Reactive sputtering, Ridge waveguides, Silicon, Sputter deposition, Cooperative upconversion, Reactive co-sputtering, Spectroscopic property, Amorphous silicon
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-290414 (URN)10.1364/CLEO_SI.2020.STh4F.4 (DOI)2-s2.0-85095407144 (Scopus ID)
Conference
CLEO: Science and Innovations, CLEO_SI 2020; Washington; United States; 10 May 2020 through 15 May 2020
Note

QC 20210322

Available from: 2021-03-22 Created: 2021-03-22 Last updated: 2022-06-25Bibliographically approved
Loiko, P., Agazzi, L., Kores, C. C., DIjkstra, M., Geskus, D. & Pollnau, M. (2020). Spectroscopy, Cooperative Upconversion and Optical Gain in Amorphous Al2O3:Yb3+ Waveguides on Silicon. In: Conference Proceedings - Lasers and Electro-Optics Society Annual Meeting-LEOS: . Paper presented at 2020 Conference on Lasers and Electro-Optics, CLEO 2020, 10 May 2020 through 15 May 2020. Institute of Electrical and Electronics Engineers Inc.
Open this publication in new window or tab >>Spectroscopy, Cooperative Upconversion and Optical Gain in Amorphous Al2O3:Yb3+ Waveguides on Silicon
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2020 (English)In: Conference Proceedings - Lasers and Electro-Optics Society Annual Meeting-LEOS, Institute of Electrical and Electronics Engineers Inc. , 2020Conference paper, Published paper (Refereed)
Abstract [en]

Ridge waveguides in amorphous Al2O3:Yb3+ are produced by reactive co-sputtering and reactive-ion etching. Their spectroscopic properties, optical gain, and cooperative upconversion are studied and explained based on a model of distinct ion classes. 

Place, publisher, year, edition, pages
Institute of Electrical and Electronics Engineers Inc., 2020
Keywords
Alumina, Aluminum oxide, Optical gain, Optical waveguides, Reactive sputtering, Ridge waveguides, Silicon, Sputter deposition, Cooperative upconversion, Reactive co-sputtering, Spectroscopic property, Amorphous silicon
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-302849 (URN)000612090003288 ()2-s2.0-85091644207 (Scopus ID)
Conference
2020 Conference on Lasers and Electro-Optics, CLEO 2020, 10 May 2020 through 15 May 2020
Note

Not duplicate with DiVA 1538950

QC 20211003

Available from: 2021-10-03 Created: 2021-10-03 Last updated: 2022-09-28Bibliographically approved
Reijn, S.-M. -., Geskus, D. & Wetter, N. U. (2019). Investigation of the geometrical depth of focus of focal spots obtained by scattering lenses operating in the transversal and lateral direction. In: Proceedings 2015 European Conference on Lasers and Electro-Optics - European Quantum Electronics Conference, CLEO/Europe-EQEC 2015: . Paper presented at 2015 European Conference on Lasers and Electro-Optics - European Quantum Electronics Conference, CLEO/Europe-EQEC 2015; International Congress Centre (ICM)Munich; Germany; 21 June 2015 through 25 June 2015. Optical Society of America
Open this publication in new window or tab >>Investigation of the geometrical depth of focus of focal spots obtained by scattering lenses operating in the transversal and lateral direction
2019 (English)In: Proceedings 2015 European Conference on Lasers and Electro-Optics - European Quantum Electronics Conference, CLEO/Europe-EQEC 2015, Optical Society of America, 2019Conference paper, Published paper (Refereed)
Place, publisher, year, edition, pages
Optical Society of America, 2019
National Category
Nano Technology
Identifiers
urn:nbn:se:kth:diva-251854 (URN)2-s2.0-85095472583 (Scopus ID)
Conference
2015 European Conference on Lasers and Electro-Optics - European Quantum Electronics Conference, CLEO/Europe-EQEC 2015; International Congress Centre (ICM)Munich; Germany; 21 June 2015 through 25 June 2015
Note

QC 20190614

Not duplicate with DiVA 1117090

Part of ISBN 9781467374750

Available from: 2019-06-14 Created: 2019-06-14 Last updated: 2024-10-25Bibliographically approved
Kores, C. C., Ismail, N., Geskus, D., Dijkstra, M., Bernhardi, E. H. & Pollnau, M. (2018). Spectral broadening in distributed-feedback resonators due to thermal chirp. In: Optics InfoBase Conference Papers: . Paper presented at Bragg Gratings, Photosensitivity and Poling in Glass Waveguides and Materials, BGPPM 2018, Zurich, Switzerland, 2 July 2018 through 5 July 2018. Optical Society of America
Open this publication in new window or tab >>Spectral broadening in distributed-feedback resonators due to thermal chirp
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2018 (English)In: Optics InfoBase Conference Papers, Optical Society of America, 2018Conference paper, Published paper (Refereed)
Abstract [en]

We investigate the spectral response of an unpumped distributed-feedback waveguide resonator, subject to thermal chirp. Experimental and simulated results indicate that such chirp causes an increase in outcoupling losses and, therefore, in the resonance linewidth.

Place, publisher, year, edition, pages
Optical Society of America, 2018
National Category
Other Engineering and Technologies
Identifiers
urn:nbn:se:kth:diva-238392 (URN)10.1364/BGPPM.2018.BTh3A.4 (DOI)2-s2.0-85051244033 (Scopus ID)9781557528209 (ISBN)
Conference
Bragg Gratings, Photosensitivity and Poling in Glass Waveguides and Materials, BGPPM 2018, Zurich, Switzerland, 2 July 2018 through 5 July 2018
Note

QC 20181108

Available from: 2018-11-08 Created: 2018-11-08 Last updated: 2024-03-15Bibliographically approved
Kores, C. C., Ismail, N., Geskus, D., Dijkstra, M., Bernhardi, E. H. & Pollnau, M. (2018). Temperature Dependence of Spectral Characteristics of Distributed-Feedback Resonators. In: Taccheo, S Mackenzie, JI Ferrari, M (Ed.), FIBER LASERS AND GLASS PHOTONICS: MATERIALS THROUGH APPLICATIONS. Paper presented at Conference on Fiber Lasers and Glass Photonics - Materials through Applications, APR 22-26, 2018, Strasbourg, FRANCE. SPIE-INT SOC OPTICAL ENGINEERING, Article ID 106830B.
Open this publication in new window or tab >>Temperature Dependence of Spectral Characteristics of Distributed-Feedback Resonators
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2018 (English)In: FIBER LASERS AND GLASS PHOTONICS: MATERIALS THROUGH APPLICATIONS / [ed] Taccheo, S Mackenzie, JI Ferrari, M, SPIE-INT SOC OPTICAL ENGINEERING , 2018, article id 106830BConference paper, Published paper (Refereed)
Abstract [en]

The spectral response of a distributed-feedback resonator with a thermal chirp is investigated. An Al2O3 channel waveguide with a surface Bragg grating inscribed into its SiO2 top cladding is studied. A linear temperature gradient along the resonator leads to a corresponding variation of the grating period. We characterize its spectral response with respect to wavelength and linewidth changes of the resonance peak. Simulated results show good agreement with the experimental data, indicating that the resonance wavelength is determined by the total accumulated phase shift. The calculated grating reflectivities at the resonance wavelength largely explain the observed changes of the resonance linewidth. This agreement demonstrates that the linewidth increase is caused by the increase of resonator outcoupling losses.

Place, publisher, year, edition, pages
SPIE-INT SOC OPTICAL ENGINEERING, 2018
Series
Proceedings of SPIE, ISSN 0277-786X ; 10683
Keywords
Distributed-feedback laser, Bragg grating, Thermal grating chirp, Resonance wavelength, Resonance linewidth
National Category
Physical Sciences
Identifiers
urn:nbn:se:kth:diva-240042 (URN)10.1117/12.2307023 (DOI)000450857500009 ()2-s2.0-85049793405 (Scopus ID)978-1-5106-1893-0 (ISBN)
Conference
Conference on Fiber Lasers and Glass Photonics - Materials through Applications, APR 22-26, 2018, Strasbourg, FRANCE
Note

QC 20181210

Available from: 2018-12-10 Created: 2018-12-10 Last updated: 2024-03-15Bibliographically approved
Calil Kores, C., Ismail, N., Geskus, D., Dijkstra, M., Bernhardi, E. H. & Pollnau, M. (2018). Temperature dependence of the resonance line of optically pumped distributed-feedback lasers. In: Optics InfoBase Conference Papers: . Paper presented at Advanced Solid State Lasers, ASSL 2018; Boston; United States; 4 November 2018 through 8 November 2018. OSA - The Optical Society
Open this publication in new window or tab >>Temperature dependence of the resonance line of optically pumped distributed-feedback lasers
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2018 (English)In: Optics InfoBase Conference Papers, OSA - The Optical Society , 2018Conference paper, Published paper (Refereed)
Abstract [en]

We characterize experimentally and theoretically a distributed-feedback laser resonator subject to a thermal chirp. The total accumulated phase shift determines the resonance wavelength. The reflectivities (outcoupling losses) at the resonance wavelength govern the resonance linewidth.

Place, publisher, year, edition, pages
OSA - The Optical Society, 2018
National Category
Other Natural Sciences
Identifiers
urn:nbn:se:kth:diva-246518 (URN)10.1364/ASSL.2018.ATh2A.26 (DOI)2-s2.0-85059485052 (Scopus ID)9781943580484 (ISBN)
Conference
Advanced Solid State Lasers, ASSL 2018; Boston; United States; 4 November 2018 through 8 November 2018
Note

QC 20190403

Available from: 2019-04-03 Created: 2019-04-03 Last updated: 2024-03-15Bibliographically approved
Calil Kores, C., Ismail, N., Geskus, D., Dijkstra, M., Bernhardi, E. & Pollnau, M. (2018). Temperature dependence of the spectral characteristics of distributed-feedback resonators. Optics Express, 26(4), 4892-4905
Open this publication in new window or tab >>Temperature dependence of the spectral characteristics of distributed-feedback resonators
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2018 (English)In: Optics Express, E-ISSN 1094-4087, Vol. 26, no 4, p. 4892-4905Article in journal (Refereed) Published
Abstract [en]

We characterize the spectral response of a distributed-feedback resonator when subject to a thermal chirp. An Al2O3 rib waveguide with a corrugated surface Bragg grating inscribed into its SiO2 top cladding is experimentally investigated. We induce a near-to-linear temperature gradient along the resonator, leading to a similar variation of the grating period, and characterize its spectral response in terms of wavelength and linewidth of the resonance peak. Simulations are carried out, showing good agreement with the experimental results and indicating that the wavelength of the resonance peak is a result only of the total accumulated phase shift. For any chirp profile we are able to calculate the reflectivities at the resonance wavelength, and this information largely explains how the linewidth of the resonance changes. This result shows that the increase in linewidth is governed by the increase of the resonator outcoupling losses. 

National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-224792 (URN)10.1364/OE.26.004892 (DOI)000426268500103 ()29475333 (PubMedID)2-s2.0-85042107476 (Scopus ID)
Note

QC 20180326

Available from: 2018-03-25 Created: 2018-03-25 Last updated: 2024-03-15Bibliographically approved
Organisations
Identifiers
ORCID iD: ORCID iD iconorcid.org/0000-0001-7895-1808

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