Open this publication in new window or tab >>Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
KTH, School of Engineering Sciences (SCI), Physics, Condensed Matter Theory.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA; CALTECH, Div Phys Math & Astron, 1200 E Calif Blvd, Pasadena, CA 91125 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.
Max Planck Inst Phys Komplexer Syst, Nothnitzer Str 38, D-01187 Dresden, Germany.
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA; Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA; CIFAR Azrieli Global Scholars Program, 661 Univ Ave, Toronto, ON M5G 1M1, Canada.
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2025 (English)In: Science Advances, E-ISSN 2375-2548, Vol. 11, no 13, article id eadn9021Article in journal (Refereed) Published
Abstract [en]
Thermalization, while ubiquitous in physics, has traditionally been viewed as an obstacle to be mitigated. In contrast, we demonstrate here the use of thermalization in the generation, control, and readout of "shell-like" spin textures with interacting 13C nuclear spins in diamond, wherein spins are polarized oppositely on either side of a critical radius. The textures span several nanometers and encompass many hundred spins; they are created and interrogated without manipulating the nuclear spins individually. Long-time stabilization is achieved via prethermalization to a Floquet-engineered Hamiltonian under the electronic gradient field: The texture is therefore metastable and robust against spin diffusion. This enables the state to endure over multiple minutes before it decays. Our work on spin-state engineering paves the way for applications in quantum simulation and nanoscale imaging.
Place, publisher, year, edition, pages
American Association for the Advancement of Science (AAAS), 2025
National Category
Condensed Matter Physics
Identifiers
urn:nbn:se:kth:diva-363140 (URN)10.1126/sciadv.adn9021 (DOI)001455518300018 ()40153504 (PubMedID)2-s2.0-105001683678 (Scopus ID)
Note
QC 20250506
2025-05-062025-05-062025-05-06Bibliographically approved