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Migration behavior of Se(IV) and Re(VII) in muscovite for potential application in deep geological nuclear waste repositories
School of Nuclear Science and Technology, University of South China, 421001, Hengyang, China; R&D and Modelling Center for Treatment and Disposal of Radioactive Waste, University of South China, 421001, Hengyang, China.
School of Nuclear Science and Technology, University of South China, 421001, Hengyang, China; R&D and Modelling Center for Treatment and Disposal of Radioactive Waste, University of South China, 421001, Hengyang, China.
School of Nuclear Science and Technology, University of South China, 421001, Hengyang, China; R&D and Modelling Center for Treatment and Disposal of Radioactive Waste, University of South China, 421001, Hengyang, China.
School of Nuclear Science and Technology, University of South China, 421001, Hengyang, China; R&D and Modelling Center for Treatment and Disposal of Radioactive Waste, University of South China, 421001, Hengyang, China.
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2024 (English)In: Journal of Radioanalytical and Nuclear Chemistry, ISSN 0236-5731, E-ISSN 1588-2780, Vol. 333, no 4, p. 2015-2026Article in journal (Refereed) Published
Abstract [en]

The migration behavior of Se(IV) and Re(VII) in muscovite was studied by capillary diffusion method and diffusion cell method. The results show that diffusion accelerates when the density decreases and the ionic strength increases. At the same time, pH also significantly affects their migration. The apparent diffusion coefficient ranges from 10–11 to 10–9 m/s2. This work can provide potential applications in deep geological nuclear waste repositories.
Place, publisher, year, edition, pages
Springer Nature , 2024. Vol. 333, no 4, p. 2015-2026
Keywords [en]
Accessible porosity, Diffusion, Muscovite, pH
National Category
Physical Chemistry
Identifiers
URN: urn:nbn:se:kth:diva-367037DOI: 10.1007/s10967-024-09427-4ISI: 001176702200001Scopus ID: 2-s2.0-85186875791OAI: oai:DiVA.org:kth-367037DiVA, id: diva2:1983642
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QC 20250711

Available from: 2025-07-11 Created: 2025-07-11 Last updated: 2025-07-11Bibliographically approved

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Liu, Longcheng

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