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Cr-Cr distance and magnetism in the phase diagram of triangular lattice antiferromagnets: A systematic comparative study
KTH, School of Engineering Sciences (SCI), Applied Physics, Materials and Nanophysics.ORCID iD: 0000-0003-4441-8882
Comprehens Res Org Sci & Soc CROSS, Neutron Sci & Technol Ctr, Tokai, Ibaraki 3191106, Japan.;Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan..
Univ Zurich, Phys Inst, Winterthurerstr 190, CH-8057 Zurich, Switzerland.; Uppsala Univ, Dept Phys & Astron, Box 516, SE-75120 Uppsala, Sweden.ORCID iD: 0000-0001-8879-7875
KEK, Inst Mat Struct Sci, Muon Sci Lab, Tokai, Ibarak 3191106, Japan..
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2024 (English)In: Physical Review Materials, E-ISSN 2475-9953, Vol. 8, no 8, article id 084403Article in journal (Refereed) Published
Abstract [en]

In this study, we investigate the influence of Cr-Cr distances on the magnetic properties of triangular lattice antiferromagnets through the lens of the recently synthesized Cr compounds LiCrSe2, 2 , LiCrTe2, 2 , and NaCrTe2. 2 . Our comprehensive analysis integrates existing magnetic structure data and new insights from muon spin rotation measurements, revealing a striking mutual influence between strongly correlated electrons and structural degrees of freedom in systems possessing very different magnetic properties despite having the same crystal symmetry. In particular, we delineate how Cr-Cr distances specifically dictate the magnetic behaviors of the triangular lattice antiferromagnets LiCrSe2, 2 , LiCrTe2, 2 , and NaCrTe2. 2 . By crafting phase diagrams based on these distances, we establish a clear correlation between the structural parameters and the magnetic ground states of these materials together with a wide variety of trivalent Cr triangular lattice layered magnets. Our analysis uncovers a transition range for in-plane and out-of-plane Cr-Cr distances that demarcates distinct magnetic behaviors, highlighting the nuanced role of lattice geometry in the spin-lattice interaction and electron correlation dynamics.

Place, publisher, year, edition, pages
American Physical Society (APS) , 2024. Vol. 8, no 8, article id 084403
National Category
Condensed Matter Physics
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URN: urn:nbn:se:kth:diva-352680DOI: 10.1103/PhysRevMaterials.8.084403ISI: 001292162800002Scopus ID: 2-s2.0-85200838862OAI: oai:DiVA.org:kth-352680DiVA, id: diva2:1895312
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QC 20240905

Available from: 2024-09-05 Created: 2024-09-05 Last updated: 2024-09-05Bibliographically approved

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Nocerino, ElisabettaForslund, Ola KenjiSassa, YasmineMånsson, Martin

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