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Ultrafast Pseudomagnetic Fields from Electron-Nuclear Quantum Geometry
Univ Hamburg, Inst Theoret Phys, Notkestr 9-11, D-22607 Hamburg, Germany..ORCID iD: 0000-0002-5453-9779
Univ Hamburg, Inst Theoret Phys, Notkestr 9-11, D-22607 Hamburg, Germany..
Univ Hamburg, Inst Theoret Phys, Notkestr 9-11, D-22607 Hamburg, Germany..
Univ Wurzburg, Inst Theoret Phys & Astrophys, D-97074 Wurzburg, Germany.;Univ Wurzburg, Wurzburg Dresden Cluster Excellence ct qmat, D-97074 Wurzburg, Germany. Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. Stockholm Univ, Nordita, Hannes Alfvens vag 12, SE-10691 Stockholm, Sweden..ORCID iD: 0000-0003-2218-2901
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2025 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 134, no 1, article id 016705Article in journal (Refereed) Published
Abstract [en]

Recent experiments demonstrate precise control over coherently excited circular phonon modes using high-intensity terahertz lasers, opening new pathways towards dynamical, ultrafast design of magnetism in functional materials. While the phonon Zeeman effect enables a theoretical description of phonon-induced magnetism, it lacks efficient angular momentum transfer from the phonon to the electron sector. In this work, we put forward a coupling mechanism based on electron-nuclear quantum geometry, with the inverse Faraday effect as a limiting case. This effect is rooted in the phase accumulation of the electronic wave function under a circular evolution of nuclear coordinates. An excitation pulse then induces a transient level splitting between electronic orbitals that carry angular momentum. First-principles simulations on SrTiO3 demonstrate that in parts of the Brillouin zone, this splitting between orbitals carrying angular momentum can easily reach 50 meV.

Place, publisher, year, edition, pages
American Physical Society (APS) , 2025. Vol. 134, no 1, article id 016705
National Category
Condensed Matter Physics
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URN: urn:nbn:se:kth:diva-359546DOI: 10.1103/PhysRevLett.134.016705ISI: 001396996100014PubMedID: 39913742Scopus ID: 2-s2.0-85214514695OAI: oai:DiVA.org:kth-359546DiVA, id: diva2:1934880
Note

QC 20250205

Available from: 2025-02-05 Created: 2025-02-05 Last updated: 2025-05-27Bibliographically approved

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Balatsky, Alexander V.

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