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Self-compression of femtosecond pulses in second-order nonlinear media and precise characterisation of ultrashort pulses
KTH, School of Engineering Sciences (SCI), Applied Physics, Light and Matter Physics. (Laser physics)ORCID iD: 0000-0001-5425-8267
2025 (English)Doctoral thesis, comprehensive summary (Other academic)
Abstract [en]

Femtosecond laser pulses are essential tools in modern science and technology, yet generating pulses that are both extremely short and experimentally accessible remains a persistent challenge. Conventional post-compression methods rely on the Kerr effect, a third-order nonlinear effect, but these approaches often require complex setups and a large laboratory footprint. This thesis explores a fundamentally different route to pulse compression by utilising the coherently driven transversal optical phonon-polariton modes in Potassium Titanyl Phosphate (KTP). Rather than relying on Kerr-based spectral broadening and subsequent dispersive compression, the method exploits strong second-order nonlinearities in KTP to generate polaritons by optical rectification so that their electric fields may be used for efficient Stokes sideband generation by electro-optic interaction. The resulting interplay with normal dispersion in the nonlinear crystal results in an order of magnitude shorter self-compressed pulses generated in a simple setup. Such pulses demand advanced characterisation methods. Building on insights from applied mathematics and optimisation theory, a new retrieval algorithm for Frequency-Resolved Optical Gating (FROG) measurements is introduced, which we call the Line-Search FROG (LSF) algorithm, that decouples the measurement data from the reconstruction process. This greatly improves the performance of the pulse retrieval fidelity in the presence of large amounts of noise. The LSF algorithm is highly versatile and applicable to all FROG geometries, including the so-called double-blind FROG, with which we managed to measure the phase of a mode-locked dark pulse for the first time. Other pulse measurement techniques such as dispersion scan could benefit as well as the underlying optimisation problem is similar. To further improve the performance of pulse characterisation techniques, we also present the Sigma Check, which is a general algorithmic step that aims to reduce the likelihood of stagnating at local minima. This is achieved by performing an image-recognition step that correctly identifies and counteracts local minimums.

Place, publisher, year, edition, pages
Stockholm: KTH Royal Institute of Technology, 2025. , p. 143
Series
TRITA-SCI-FOU ; 2025:33
National Category
Atom and Molecular Physics and Optics
Research subject
Physics, Optics and Photonics
Identifiers
URN: urn:nbn:se:kth:diva-368178ISBN: 978-91-8106-358-5 (electronic)OAI: oai:DiVA.org:kth-368178DiVA, id: diva2:1987546
Public defence
2025-08-22, Pärlan, Albanovägen 26, Stockholm, 10:00 (English)
Opponent
Supervisors
Note

QC 2025-08-11

Available from: 2025-08-11 Created: 2025-08-06 Last updated: 2025-08-18Bibliographically approved
List of papers
1. Overcoming noise in pulse retrieval: introducing the line-search FROG algorithm
Open this publication in new window or tab >>Overcoming noise in pulse retrieval: introducing the line-search FROG algorithm
2025 (English)In: Optics Express, E-ISSN 1094-4087, Vol. 33, no 16, article id 33258Article in journal (Refereed) Published
Abstract [en]

The most widely used frequency-resolved optical gating (FROG) retrieval algorithm solves the trace inversion problem to retrieve the phase distribution of the ultrashort pulse electric field by using preprocessed measured data in each iterative step to improve subsequent guesses. Such algorithms work very well for measurements with high signal-to-noise ratios but can become less reliable in extracting weaker signals buried in noisy data. We introduce the line-search FROG (LSF) algorithm, which enhances noise robustness by treating measurement data passively, using it solely for error evaluation rather than iterative correction. The gradient-free LSF algorithm requires no preprocessing of the measurement data and thus does not make assumptions about the noise in the measured traces. We show that LSF achieves comparable FROG error metrics to a ptychographic retrieval algorithm and COPRA, while producing higher-quality pulse reconstructions with reduced noise contaminations. It is applicable to all FROG geometries, supports blind FROG retrieval, and can reconstruct pulses from incomplete datasets.

Place, publisher, year, edition, pages
Optica Publishing Group, 2025
National Category
Physical Sciences
Research subject
Physics, Optics and Photonics
Identifiers
urn:nbn:se:kth:diva-368060 (URN)10.1364/oe.569606 (DOI)001551837300005 ()2-s2.0-105013098631 (Scopus ID)
Funder
Swedish Research Council, 2023-04985
Note

QC 20250805

Available from: 2025-08-04 Created: 2025-08-04 Last updated: 2025-12-08Bibliographically approved
2. Avoiding local minima in FROG retrievals with a convergence evaluation metric
Open this publication in new window or tab >>Avoiding local minima in FROG retrievals with a convergence evaluation metric
2025 (English)In: Applied Optics, ISSN 1559-128X, E-ISSN 2155-3165, Vol. 64, no 19, p. 5558-5558Article in journal (Refereed) Published
Abstract [en]

Accurate retrieval of ultrashort laser pulses using frequency-resolved optical gating (FROG) is often hindered bylocal convergence in existing algorithms. We introduce the Sigma Check, a novel supervised evaluation step, to ourknowledge, designed to detect and mitigate erroneous convergence to local minima. This method evaluates thedifference between measured and retrieved spectrograms, applying targeted perturbation when significant discrepancies are detected. Numerical simulations and experimental measurements demonstrate that the Sigma Checkenhances retrieval accuracy across multiple algorithms, including line-search FROG, extended ptychographiciterative engine, and principal components generalized projections algorithm, providing a systematic approach toimproving FROG pulse reconstruction.

Place, publisher, year, edition, pages
Optica Publishing Group, 2025
National Category
Natural Sciences Physical Sciences
Research subject
Physics, Optics and Photonics
Identifiers
urn:nbn:se:kth:diva-368059 (URN)10.1364/ao.564293 (DOI)001524140000041 ()2-s2.0-105010562077 (Scopus ID)
Funder
Swedish Research Council, 2023-04985Carl Tryggers foundation , CTS23:2795
Note

QC 20250805

Available from: 2025-08-04 Created: 2025-08-04 Last updated: 2025-08-06Bibliographically approved
3. Generation of femtosecond pulse bursts at multiple-THz repetition rate by nonlinear self-compression in bulk KTP
Open this publication in new window or tab >>Generation of femtosecond pulse bursts at multiple-THz repetition rate by nonlinear self-compression in bulk KTP
2024 (English)In: 11th EPS-QEOD Europhoton Conference on Solid-State, Fibre, and Waveguide Coherent Light Sources, EUROPHOTON 2024, EDP Sciences , 2024, article id 04064Conference paper, Published paper (Refereed)
Abstract [en]

A chirped 470 fs pulse at 1030 nm was used to generate a phonon-polariton wave in bulk KTP by optical rectification. Phase modulation of the pump by the polariton wave resulted in generation of a burst of 20 fs pulses.

Place, publisher, year, edition, pages
EDP Sciences, 2024
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-358221 (URN)10.1051/epjconf/202430704064 (DOI)2-s2.0-85212853206 (Scopus ID)
Conference
11th EPS-QEOD Europhoton Conference on Solid-State, Fibre, and Waveguide Coherent Light Sources, EUROPHOTON 2024, Vilnius, Lithuania, Aug 25 2024 - Aug 30 2024
Note

QC 20250114

Available from: 2025-01-07 Created: 2025-01-07 Last updated: 2025-08-06Bibliographically approved
4. Self-Compression in Single-Domain KTP at 1 micron in a Normal Dispersion Regime
Open this publication in new window or tab >>Self-Compression in Single-Domain KTP at 1 micron in a Normal Dispersion Regime
Show others...
2022 (English)In: Optics InfoBase Conference Papers, Optica Publishing Group (formerly OSA) , 2022, article id SM3O.2Conference paper, Published paper (Refereed)
Abstract [en]

We demonstrate self-compression of 173 fs pulses centered at 1030 nm down to 19.5 fs through electro-optic phase modulation by the phonon-polariton waves generated in a phase-matched intra-pulse difference-frequency mixing.

Place, publisher, year, edition, pages
Optica Publishing Group (formerly OSA), 2022
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-329729 (URN)2-s2.0-85136802991 (Scopus ID)
Conference
CLEO: Applications and Technology, A and T 2022, San Jose, CA, USA, 15-20 May 2022
Note

Part of ISBN 9781557528209

Syskonpost

Not duplicate with DiVA 1763546

QC 20230622

Available from: 2023-06-22 Created: 2023-06-22 Last updated: 2025-08-06Bibliographically approved
5. Self-Compression in Single-Domain KTP at 1 micron in a Normal Dispersion Regime
Open this publication in new window or tab >>Self-Compression in Single-Domain KTP at 1 micron in a Normal Dispersion Regime
Show others...
2022 (English)In: 2022 Conference on Lasers and Electro-Optics, CLEO 2022: Proceedings, Institute of Electrical and Electronics Engineers Inc. , 2022Conference paper, Published paper (Refereed)
Abstract [en]

We demonstrate self-compression of 173 fs pulses centered at 1030 nm down to 19.5 fs through electro-optic phase modulation by the phonon-polariton waves generated in a phase-matched intra-pulse difference-frequency mixing.

Place, publisher, year, edition, pages
Institute of Electrical and Electronics Engineers Inc., 2022
Keywords
Phase matching, Difference-frequency mixing, Electro-optic phase, Fs-pulses, Normal dispersion, Phonon polaritons, Self-compression, Single domains, Phonons
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-328158 (URN)2-s2.0-85139942526 (Scopus ID)
Conference
2022 Conference on Lasers and Electro-Optics, CLEO 2022, 15-20 May 2022
Note

QC 20230607

Available from: 2023-06-07 Created: 2023-06-07 Last updated: 2025-08-06Bibliographically approved
6. Eliminating local convergences in FROG retrieval algorithms
Open this publication in new window or tab >>Eliminating local convergences in FROG retrieval algorithms
2023 (English)In: EPJ Web of Conferences, EDP Sciences , 2023, Vol. 287, article id 08001Conference paper, Oral presentation with published abstract (Refereed)
Place, publisher, year, edition, pages
EDP Sciences, 2023
National Category
Physical Sciences
Research subject
Physics, Optics and Photonics
Identifiers
urn:nbn:se:kth:diva-368062 (URN)10.1051/epjconf/202328708001 (DOI)
Conference
European Optical Society Annual Meeting (EOSAM) 2023
Note

QC 20250806

Available from: 2025-08-04 Created: 2025-08-04 Last updated: 2025-08-06Bibliographically approved
7. Experimental study of the pump configuration's impact on gain-managed nonlinear amplification in an Yb-doped fiber amplifier
Open this publication in new window or tab >>Experimental study of the pump configuration's impact on gain-managed nonlinear amplification in an Yb-doped fiber amplifier
2021 (English)In: Optics InfoBase Conference Papers, The Optical Society , 2021Conference paper, Published paper (Refereed)
Place, publisher, year, edition, pages
The Optical Society, 2021
National Category
Other Physics Topics
Identifiers
urn:nbn:se:kth:diva-313451 (URN)2-s2.0-85166461328 (Scopus ID)
Conference
2021 European Conference on Lasers and Electro-Optics, CLEO/Europe 2021, Virtual/Online, 21 June 2021 through 25 June 2021
Note

QC 20220603

Part of proceedings: ISBN 978-155752820-9 

Not duplicate with DiVA 1637512

Available from: 2022-06-03 Created: 2022-06-03 Last updated: 2025-08-06Bibliographically approved
8. Experimental study of the pump configuration's impact on gain-managed nonlinear amplification in an Yb-doped fiber amplifier
Open this publication in new window or tab >>Experimental study of the pump configuration's impact on gain-managed nonlinear amplification in an Yb-doped fiber amplifier
2021 (English)In: 2021 Conference On Lasers And Electro-Optics Europe & European Quantum Electronics Conference (CLEO/EUROPE-EQEC), Institute of Electrical and Electronics Engineers (IEEE) , 2021Conference paper, Published paper (Refereed)
Place, publisher, year, edition, pages
Institute of Electrical and Electronics Engineers (IEEE), 2021
National Category
Telecommunications Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-308791 (URN)10.1109/CLEO/Europe-EQEC52157.2021.9542331 (DOI)000728078300695 ()2-s2.0-85117613884 (Scopus ID)
Conference
Conference on Lasers and Electro-Optics Europe / European Quantum Electronics Conference (CLEO/Europe-EQEC), JUN 21-25, 2021, ELECTR NETWORK
Note

Part of proceedings: ISBN 978-1-6654-1876-8

QC 20220214

Available from: 2022-02-14 Created: 2022-02-14 Last updated: 2025-08-06Bibliographically approved
9. Line-search FROG algorithm for retrieval of pulses from noisy datasets
Open this publication in new window or tab >>Line-search FROG algorithm for retrieval of pulses from noisy datasets
2022 (English)In: EPJ Web of Conferences, EDP Sciences , 2022, Vol. 267, article id 01051Conference paper, Oral presentation with published abstract (Refereed)
Place, publisher, year, edition, pages
EDP Sciences, 2022
National Category
Physical Sciences
Research subject
Physics, Optics and Photonics
Identifiers
urn:nbn:se:kth:diva-368061 (URN)10.1051/epjconf/202226701051 (DOI)
Conference
Europhoton 2022
Note

QC 20250806

Available from: 2025-08-04 Created: 2025-08-04 Last updated: 2025-08-06Bibliographically approved
10. Intra-cavity dark pulse generation through synchronized sum-frequency mixing
Open this publication in new window or tab >>Intra-cavity dark pulse generation through synchronized sum-frequency mixing
Show others...
2022 (English)In: Optics Letters, ISSN 0146-9592, E-ISSN 1539-4794, Vol. 47, no 5, p. 1105-1108Article in journal (Refereed) Published
Abstract [en]

A Nd:YVO4 laser operating at 1064 nm generating a stable mode-locked train of 10 ps-long dark pulses with a 211 MHz repetition rate is presented. The mode-locking relies on a periodic loss modulation produced by intra-cavity sum-frequency mixing with a synchronous bright-pulse train from a mode-locked femtosecond Yb:KYW laser at 1040 nm. A modulation depth of 9050 was achieved for the dark pulses, confirmed by cross-correlation measurements. The ultrafast loss modulation injects power into the Nd:YVO4 laser cavity modes beyond the laser gain bandwidth. At proper laser cavity length, the detuning interaction of these modes with the lasing modes leads to the generation of periodic ultra-fast transients at frequencies above 1.5 THz.

Place, publisher, year, edition, pages
Optica Publishing Group, 2022
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-310258 (URN)10.1364/OL.448148 (DOI)000762499000024 ()35230302 (PubMedID)2-s2.0-85125180302 (Scopus ID)
Note

QC 20220328

Available from: 2022-03-28 Created: 2022-03-28 Last updated: 2025-08-06Bibliographically approved
11. The phase of darkness - measuring the phase of a dark pulse
Open this publication in new window or tab >>The phase of darkness - measuring the phase of a dark pulse
2024 (English)In: EOS ANNUAL MEETING, EOSAM 2024 / [ed] DeStefano, L Velotta, R Descrovi, E, EDP Sciences , 2024, Vol. 309, p. 07014-, article id 07014Conference paper, Published paper (Refereed)
Abstract [en]

Dark optical solitons are solutions to the nonlinear Schrodinger equation in normal dispersion media with positive Kerr nonlinearity, exhibiting a discrete pi phase jump. These solitons are valuable to applications within telecommunication. Recent advancements have demonstrated the generation of two-colour bright-dark soliton pairs through cross-amplitude modulation in laser cavities, resulting in mode locking. In this study we present for the first time full field characterization of the electric field of a dark pulse. We achieved this by performing Blind Frequency Resolved Optical Gating measurements using the synchronous bright pulse as the gate pulse. The retrieved dark pulse verifies the existence of the expected p phase jump in the phase of the dark pulse, confirming theoretical predictions.

Place, publisher, year, edition, pages
EDP Sciences, 2024
Series
EPJ Web of Conferences, ISSN 2100-014X
National Category
Atom and Molecular Physics and Optics
Identifiers
urn:nbn:se:kth:diva-360735 (URN)10.1051/epjconf/202430907014 (DOI)001353751800132 ()2-s2.0-85212478513 (Scopus ID)
Conference
EOS Annual Meeting (EOSAM), SEP 09-13, 2024, Naples, ITALY
Note

QC 20250303

Available from: 2025-03-03 Created: 2025-03-03 Last updated: 2025-08-06Bibliographically approved

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Oxelmark Krook, Christoffer

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